Articles | Volume 24, issue 4
https://doi.org/10.5194/hess-24-2105-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/hess-24-2105-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Age and origin of leaf wax n-alkanes in fluvial sediment–paleosol sequences and implications for paleoenvironmental reconstructions
Marcel Bliedtner
CORRESPONDING AUTHOR
Institute of Geography, Friedrich Schiller University of Jena,
Löbdergraben 32, 07743 Jena, Germany
Institute of Geography and Oeschger Centre for Climate Change
Research, University of Bern, 3012 Bern, Switzerland
Hans von Suchodoletz
Institute of Geography, University of Technology Dresden, 01069
Dresden, Germany
Institute of Geography, University of Leipzig, 04103 Leipzig, Germany
Imke Schäfer
Institute of Geography and Oeschger Centre for Climate Change
Research, University of Bern, 3012 Bern, Switzerland
Caroline Welte
Laboratory of Ion Beam Physics, ETH Zurich, 8093 Zurich, Switzerland
Gary Salazar
Department of Chemistry and Biochemistry and Oeschger Centre for
Climate Change Research, University of Bern, 3012 Bern, Switzerland
Sönke Szidat
Department of Chemistry and Biochemistry and Oeschger Centre for
Climate Change Research, University of Bern, 3012 Bern, Switzerland
Mischa Haas
Department of Surface Waters Research and Management, Eawag, 8600
Dübendorf, Switzerland
Nathalie Dubois
Department of Earth Sciences, ETH Zürich, 8006 Zurich,
Switzerland
Roland Zech
Institute of Geography, Friedrich Schiller University of Jena,
Löbdergraben 32, 07743 Jena, Germany
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Karl Espen Yttri, David Simpson, Robert Bergström, Gyula Kiss, Sönke Szidat, Darius Ceburnis, Sabine Eckhardt, Christoph Hueglin, Jacob Klenø Nøjgaard, Cinzia Perrino, Ignazio Pisso, Andre Stephan Henry Prevot, Jean-Philippe Putaud, Gerald Spindler, Milan Vana, Yan-Lin Zhang, and Wenche Aas
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Arineh Cholakian, Matthias Beekmann, Augustin Colette, Isabelle Coll, Guillaume Siour, Jean Sciare, Nicolas Marchand, Florian Couvidat, Jorge Pey, Valerie Gros, Stéphane Sauvage, Vincent Michoud, Karine Sellegri, Aurélie Colomb, Karine Sartelet, Helen Langley DeWitt, Miriam Elser, André S. H. Prévot, Sonke Szidat, and François Dulac
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Carbonaceous aerosols are related to adverse human health effects, which depend on the aerosol chemical composition and size. Here, we combine aerosol mass spectrometry and radiocarbon measurements of size-resolved samples collected over a long term to identify the origins of primary and secondary carbonaceous aerosols in the fine and coarse modes.
Di Liu, Matthias Vonwiller, Jun Li, Junwen Liu, Sönke Szidat, Yanlin Zhang, Chongguo Tian, Yinjun Chen, Zhineng Cheng, Guangcai Zhong, Pingqing Fu, and Gan Zhang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2018-295, https://doi.org/10.5194/acp-2018-295, 2018
Revised manuscript not accepted
Yan-Lin Zhang, Imad El-Haddad, Ru-Jin Huang, Kin-Fai Ho, Jun-Ji Cao, Yongming Han, Peter Zotter, Carlo Bozzetti, Kaspar R. Daellenbach, Jay G. Slowik, Gary Salazar, André S. H. Prévôt, and Sönke Szidat
Atmos. Chem. Phys., 18, 4005–4017, https://doi.org/10.5194/acp-18-4005-2018, https://doi.org/10.5194/acp-18-4005-2018, 2018
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Here we present a quantitative source apportionment of WSOC, isolated from aerosols in China using radiocarbon (14C) and offline high-resolution time of flight aerosol mass spectrometer measurements. We demonstrate a dominant contribution of non-fossil emissions to WSOC aerosols in the Northern Hemisphere. However, the fossil fraction is substantially larger in aerosols from East Asia and the east Asian pollution outflow, especially during winter, due to increasing coal combustion.
Kaspar R. Daellenbach, Imad El-Haddad, Lassi Karvonen, Athanasia Vlachou, Joel C. Corbin, Jay G. Slowik, Maarten F. Heringa, Emily A. Bruns, Samuel M. Luedin, Jean-Luc Jaffrezo, Sönke Szidat, Andrea Piazzalunga, Raquel Gonzalez, Paola Fermo, Valentin Pflueger, Guido Vogel, Urs Baltensperger, and André S. H. Prévôt
Atmos. Chem. Phys., 18, 2155–2174, https://doi.org/10.5194/acp-18-2155-2018, https://doi.org/10.5194/acp-18-2155-2018, 2018
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A novel offline LDI-MS method was developed to analyse particulate matter (PM) collected at multiple sites in central Europe during the entire year of 2013. PM sources were identified by positive matrix factorization. Wood burning emissions were separated according to the burning conditions; inefficient burns had a larger impact on air quality in southern Alpine valleys than in northern Switzerland. Moreover, primary tailpipe exhaust was distinguished from aged/secondary traffic emissions.
Julian Struck, Christopher B. Roettig, Dominik Faust, and Roland Zech
E&G Quaternary Sci. J., 66, 109–114, https://doi.org/10.5194/egqsj-66-109-2018, https://doi.org/10.5194/egqsj-66-109-2018, 2018
Marcel Lerch, Marcel Bliedtner, Christopher-Bastian Roettig, Jan-Uwe Schmidt, Sönke Szidat, Gary Salazar, Roland Zech, Bruno Glaser, Arno Kleber, and Michael Zech
E&G Quaternary Sci. J., 66, 103–108, https://doi.org/10.5194/egqsj-66-103-2018, https://doi.org/10.5194/egqsj-66-103-2018, 2018
Lorenz Wüthrich, Marcel Bliedtner, Imke Kathrin Schäfer, Jana Zech, Fatemeh Shajari, Dorian Gaar, Frank Preusser, Gary Salazar, Sönke Szidat, and Roland Zech
E&G Quaternary Sci. J., 66, 91–100, https://doi.org/10.5194/egqsj-66-91-2017, https://doi.org/10.5194/egqsj-66-91-2017, 2017
Lorenz Wüthrich, Claudio Brändli, Régis Braucher, Heinz Veit, Negar Haghipour, Carla Terrizzano, Marcus Christl, Christian Gnägi, and Roland Zech
E&G Quaternary Sci. J., 66, 57–68, https://doi.org/10.5194/egqsj-66-57-2017, https://doi.org/10.5194/egqsj-66-57-2017, 2017
S. Nemiah Ladd, Nathalie Dubois, and Carsten J. Schubert
Biogeosciences, 14, 3979–3994, https://doi.org/10.5194/bg-14-3979-2017, https://doi.org/10.5194/bg-14-3979-2017, 2017
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Hydrogen isotopes of lipids provide valuable information about microbial activity, climate, and environmental stress. We show that heavy hydrogen in fatty acids declines from spring to summer in a nutrient-rich and a nutrient-poor lake and that the effect is nearly 3 times as big in the former. This effect is likely a combination of increased biomass from algae, warmer temperatures, and higher algal growth rates.
Tesfaye A. Berhanu, Sönke Szidat, Dominik Brunner, Ece Satar, Rüdiger Schanda, Peter Nyfeler, Michael Battaglia, Martin Steinbacher, Samuel Hammer, and Markus Leuenberger
Atmos. Chem. Phys., 17, 10753–10766, https://doi.org/10.5194/acp-17-10753-2017, https://doi.org/10.5194/acp-17-10753-2017, 2017
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Fossil fuel CO2 is the major contributor of anthropogenic CO2 in the atmosphere, and accurate quantification is essential to better understand the carbon cycle. Such accurate quantification can be conducted based on radiocarbon measurements. In this study, we present radiocarbon measurements from a tall tower site in Switzerland. From these measurements, we have observed seasonally varying fossil fuel CO2 contributions and a biospheric CO2 component that varies diurnally and seasonally.
Prettiny K. Ma, Yunliang Zhao, Allen L. Robinson, David R. Worton, Allen H. Goldstein, Amber M. Ortega, Jose L. Jimenez, Peter Zotter, André S. H. Prévôt, Sönke Szidat, and Patrick L. Hayes
Atmos. Chem. Phys., 17, 9237–9259, https://doi.org/10.5194/acp-17-9237-2017, https://doi.org/10.5194/acp-17-9237-2017, 2017
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Airborne particulate matter (PM) negatively impacts air quality in cities throughout the world. An important fraction of PM is organic aerosol. We have evaluated and developed several new models for secondary organic aerosol (SOA), which is formed from the chemical processing of gaseous precursors. Using our model results, we have quantified important SOA sources and precursors and also identified possible model parameterizations that could be used for air quality predictions.
Vincent Michoud, Jean Sciare, Stéphane Sauvage, Sébastien Dusanter, Thierry Léonardis, Valérie Gros, Cerise Kalogridis, Nora Zannoni, Anaïs Féron, Jean-Eudes Petit, Vincent Crenn, Dominique Baisnée, Roland Sarda-Estève, Nicolas Bonnaire, Nicolas Marchand, H. Langley DeWitt, Jorge Pey, Aurélie Colomb, François Gheusi, Sonke Szidat, Iasonas Stavroulas, Agnès Borbon, and Nadine Locoge
Atmos. Chem. Phys., 17, 8837–8865, https://doi.org/10.5194/acp-17-8837-2017, https://doi.org/10.5194/acp-17-8837-2017, 2017
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The ChArMEx SOP2 field campaign took place from 15 July to 5 August 2013 in the western Mediterranean Basin at Ersa, a remote site in Cape Corse. Exhaustive descriptions of the chemical composition of air masses in gas and aerosol phase were performed. An analysis of these measurements was performed using various source-receptor approaches. This led to the identification of several factors linked to primary sources but also to secondary processes of both biogenic and anthropogenic origin.
Célia J. Sapart, Natalia Shakhova, Igor Semiletov, Joachim Jansen, Sönke Szidat, Denis Kosmach, Oleg Dudarev, Carina van der Veen, Matthias Egger, Valentine Sergienko, Anatoly Salyuk, Vladimir Tumskoy, Jean-Louis Tison, and Thomas Röckmann
Biogeosciences, 14, 2283–2292, https://doi.org/10.5194/bg-14-2283-2017, https://doi.org/10.5194/bg-14-2283-2017, 2017
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The Arctic Ocean, especially the Siberian shelves, overlays large areas of subsea permafrost that is degrading. We show that methane with a biogenic origin is emitted from this permafrost. At locations where bubble plumes have been observed, methane can escape oxidation in the surface sediment and rapidly migrate through the very shallow water column of this region to escape to the atmosphere, generating a positive radiative feedback.
Peter Zotter, Hanna Herich, Martin Gysel, Imad El-Haddad, Yanlin Zhang, Griša Močnik, Christoph Hüglin, Urs Baltensperger, Sönke Szidat, and André S. H. Prévôt
Atmos. Chem. Phys., 17, 4229–4249, https://doi.org/10.5194/acp-17-4229-2017, https://doi.org/10.5194/acp-17-4229-2017, 2017
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Most studies use a single Ångström exponent for wood burning (αWB) and traffic (αTR) emissions in the Aethalometer model, used for source apportionment of black carbon, derived from previous work. However, accurate determination of the α values is currently lacking. Comparing radiocarbon measurements (14C) with the Aehtalometer model, good agreement was found, indicating that the Aethalometer model reproduces reasonably well the 14C results using our best estimate of a single αWB and αTR.
Ulrike Dusek, Regina Hitzenberger, Anne Kasper-Giebl, Magdalena Kistler, Harro A. J. Meijer, Sönke Szidat, Lukas Wacker, Rupert Holzinger, and Thomas Röckmann
Atmos. Chem. Phys., 17, 3233–3251, https://doi.org/10.5194/acp-17-3233-2017, https://doi.org/10.5194/acp-17-3233-2017, 2017
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Measurements of the radioactive carbon isotope 14C allow to identify the sources of aerosol carbon. We report an extensive 14C source apportionment record in the Netherlands with samples covering a whole year. We discovered that long-range transport has a large influence on aerosol carbon levels. Fossil fuel carbon is least influenced by long-range transport and more regional in origin. Biomass burning seems to be a minor source of aerosol carbon in the Netherlands.
Chiara Uglietti, Alexander Zapf, Theo Manuel Jenk, Michael Sigl, Sönke Szidat, Gary Salazar, and Margit Schwikowski
The Cryosphere, 10, 3091–3105, https://doi.org/10.5194/tc-10-3091-2016, https://doi.org/10.5194/tc-10-3091-2016, 2016
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A meaningful interpretation of the climatic history contained in ice cores requires a precise chronology. For dating the older and deeper part of the glaciers, radiocarbon analysis can be used when organic matter such as plant or insect fragments are found in the ice. Since this happens rarely, a complementary dating tool, based on radiocarbon dating of the insoluble fraction of carbonaceous aerosols entrapped in the ice, allows for ice dating between 200 and more than 10 000 years.
Jianzhong Xu, Jinsen Shi, Qi Zhang, Xinlei Ge, Francesco Canonaco, André S. H. Prévôt, Matthias Vonwiller, Sönke Szidat, Jinming Ge, Jianmin Ma, Yanqing An, Shichang Kang, and Dahe Qin
Atmos. Chem. Phys., 16, 14937–14957, https://doi.org/10.5194/acp-16-14937-2016, https://doi.org/10.5194/acp-16-14937-2016, 2016
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This study deployed an AMS field study in Lanzhou, a city in northwestern China, evaluating the chemical composition, sources, and processes of urban aerosols during wintertime. In comparison with the results during summer in Lanzhou, the air pollution during winter was more severe and the sources were more complex. In addition, this paper estimates the contributions of fossil and non-fossil sources of organic carbon to primary and secondary organic carbon using the carbon isotopic method.
Vidmantas Ulevicius, Steigvilė Byčenkienė, Carlo Bozzetti, Athanasia Vlachou, Kristina Plauškaitė, Genrik Mordas, Vadimas Dudoitis, Gülcin Abbaszade, Vidmantas Remeikis, Andrius Garbaras, Agne Masalaite, Jan Blees, Roman Fröhlich, Kaspar R. Dällenbach, Francesco Canonaco, Jay G. Slowik, Josef Dommen, Ralf Zimmermann, Jürgen Schnelle-Kreis, Gary A. Salazar, Konstantinos Agrios, Sönke Szidat, Imad El Haddad, and André S. H. Prévôt
Atmos. Chem. Phys., 16, 5513–5529, https://doi.org/10.5194/acp-16-5513-2016, https://doi.org/10.5194/acp-16-5513-2016, 2016
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In early spring the Baltic region is frequently affected by high pollution events due to biomass burning in that area. Here we present a comprehensive study to investigate the impact of biomass/grass burning (BB) on the evolution and composition of aerosol in Preila, Lithuania, during springtime open fires.
Junwen Liu, Jun Li, Di Liu, Ping Ding, Chengde Shen, Yangzhi Mo, Xinming Wang, Chunling Luo, Zhineng Cheng, Sönke Szidat, Yanlin Zhang, Yingjun Chen, and Gan Zhang
Atmos. Chem. Phys., 16, 2985–2996, https://doi.org/10.5194/acp-16-2985-2016, https://doi.org/10.5194/acp-16-2985-2016, 2016
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Many Chinese cities now are suffering the high loadings of fine particular matters, which can bring a lot of negative impacts on air quality, human health, and the climate system. The Chinese government generally focuses on the control of the emissions from vehicles and industry. Our results evidently show that the burning of biomass materials such as wood and agricultural residues can lead to the urban air pollution in China. The characteristic of haze covering China is distinct from regions.
K. R. Daellenbach, C. Bozzetti, A. Křepelová, F. Canonaco, R. Wolf, P. Zotter, P. Fermo, M. Crippa, J. G. Slowik, Y. Sosedova, Y. Zhang, R.-J. Huang, L. Poulain, S. Szidat, U. Baltensperger, I. El Haddad, and A. S. H. Prévôt
Atmos. Meas. Tech., 9, 23–39, https://doi.org/10.5194/amt-9-23-2016, https://doi.org/10.5194/amt-9-23-2016, 2016
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In this study, we developed an offline technique using the AMS for the characterization of the chemical fingerprints of aerosols collected on quartz filters, and evaluated the suitability of the organic mass spectral data for source apportionment. This technique may be used to enhance the AMS capabilities in measuring size-fractionated, spatially resolved long-term data sets.
G. O. Mouteva, S. M. Fahrni, G. M. Santos, J. T. Randerson, Y.-L. Zhang, S. Szidat, and C. I. Czimczik
Atmos. Meas. Tech., 8, 3729–3743, https://doi.org/10.5194/amt-8-3729-2015, https://doi.org/10.5194/amt-8-3729-2015, 2015
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We describe a stepwise uncertainty analysis of 14C measurements of organic (OC) and elemental (EC) carbon fractions of aerosols. Using the Swiss_4S thermal-optical protocol with a newly established trapping setup, we show that we can efficiently isolate and trap each carbon fraction and perform 14C analysis of ultra-small OC and EC samples with high accuracy and low 14C blanks. Our study presents a first step towards the development of a common protocol for OC and EC 14C measurements.
P. L. Hayes, A. G. Carlton, K. R. Baker, R. Ahmadov, R. A. Washenfelder, S. Alvarez, B. Rappenglück, J. B. Gilman, W. C. Kuster, J. A. de Gouw, P. Zotter, A. S. H. Prévôt, S. Szidat, T. E. Kleindienst, J. H. Offenberg, P. K. Ma, and J. L. Jimenez
Atmos. Chem. Phys., 15, 5773–5801, https://doi.org/10.5194/acp-15-5773-2015, https://doi.org/10.5194/acp-15-5773-2015, 2015
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(1) Four different parameterizations for the formation and chemical evolution of secondary organic aerosol (SOA) are evaluated using a box model representing the Los Angeles region during the CalNex campaign.
(2) The SOA formed only from the oxidation of VOCs is insufficient to explain the observed SOA concentrations.
(3) The amount of SOA mass formed from diesel vehicle emissions is estimated to be 16-27%.
(4) Modeled SOA depends strongly on the P-S/IVOC volatility distribution.
J. P. Krüger, J. Leifeld, S. Glatzel, S. Szidat, and C. Alewell
Biogeosciences, 12, 2861–2871, https://doi.org/10.5194/bg-12-2861-2015, https://doi.org/10.5194/bg-12-2861-2015, 2015
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Biogeochemical soil parameters are studied to detect peatland degradation along a land use gradient (intensive, extensive, near-natural). Stable carbon isotopes, radiocarbon ages and ash content confirm peat growth in the near-natural bog but also indicate previous degradation. When the bog is managed extensively or intensively as grassland, all parameters indicate degradation and substantial C loss of the order of 18.8 to 42.9 kg C m-2.
L. R. Crilley, W. J. Bloss, J. Yin, D. C. S. Beddows, R. M. Harrison, J. D. Allan, D. E. Young, M. Flynn, P. Williams, P. Zotter, A. S. H. Prevot, M. R. Heal, J. F. Barlow, C. H. Halios, J. D. Lee, S. Szidat, and C. Mohr
Atmos. Chem. Phys., 15, 3149–3171, https://doi.org/10.5194/acp-15-3149-2015, https://doi.org/10.5194/acp-15-3149-2015, 2015
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Wood is a renewable fuel but its combustion for residential heating releases a number of locally acting air pollutants, most notably particulate matter known to have adverse effects on human health. This paper used chemical tracers for wood smoke to estimate the contribution that burning wood makes to concentrations of airborne particles in the atmosphere of southern England and most particularly in London.
Y.-L. Zhang, R.-J. Huang, I. El Haddad, K.-F. Ho, J.-J. Cao, Y. Han, P. Zotter, C. Bozzetti, K. R. Daellenbach, F. Canonaco, J. G. Slowik, G. Salazar, M. Schwikowski, J. Schnelle-Kreis, G. Abbaszade, R. Zimmermann, U. Baltensperger, A. S. H. Prévôt, and S. Szidat
Atmos. Chem. Phys., 15, 1299–1312, https://doi.org/10.5194/acp-15-1299-2015, https://doi.org/10.5194/acp-15-1299-2015, 2015
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Source apportionment of fine carbonaceous aerosols using radiocarbon and other organic markers measurements during 2013 winter haze episodes was conducted at four megacities in China. Our results demonstrate that fossil emissions predominate EC with a mean contribution of 75±8%, whereas non-fossil sources account for 55±10% of OC; and the increment of TC on heavily polluted days was mainly driven by the increase of secondary OC from both fossil-fuel and non-fossil emissions.
P. Zotter, V. G. Ciobanu, Y. L. Zhang, I. El-Haddad, M. Macchia, K. R. Daellenbach, G. A. Salazar, R.-J. Huang, L. Wacker, C. Hueglin, A. Piazzalunga, P. Fermo, M. Schwikowski, U. Baltensperger, S. Szidat, and A. S. H. Prévôt
Atmos. Chem. Phys., 14, 13551–13570, https://doi.org/10.5194/acp-14-13551-2014, https://doi.org/10.5194/acp-14-13551-2014, 2014
Related subject area
Subject: Ecohydrology | Techniques and Approaches: Theory development
Temporal shift in groundwater fauna in southwestern Germany
Root zone in the Earth system
Future response of ecosystem water use efficiency to CO2 effects in the Yellow River Basin, China
Combined impacts of climate change and human activities on blue and green water resources in the high-intensity development watershed
Soil water sources and their implications for vegetation restoration in the Three-Rivers Headwater Region during different ablation periods
Canopy structure modulates the sensitivity of subalpine forest stands to interannual snowpack and precipitation variability
Biocrust-reduced soil water retention and soil infiltration in an alpine Kobresia meadow
The natural abundance of stable water isotopes method may overestimate deep-layer soil water use by trees
Contribution of cryosphere to runoff in the transition zone between the Tibetan Plateau and arid region based on environmental isotopes
Vegetation optimality explains the convergence of catchments on the Budyko curve
Differential response of plant transpiration to uptake of rainwater-recharged soil water for dominant tree species in the semiarid Loess Plateau
Isotopic offsets between bulk plant water and its sources are larger in cool and wet environments
Hydrology without dimensions
Long-term climate-influenced land cover change in discontinuous permafrost peatland complexes
Groundwater fauna in an urban area – natural or affected?
Seasonal partitioning of precipitation between streamflow and evapotranspiration, inferred from end-member splitting analysis
The influence of litter crusts on soil properties and hydrological processes in a sandy ecosystem
Unexplained hydrogen isotope offsets complicate the identification and quantification of tree water sources in a riparian forest
A synthesis of three decades of hydrological research at Scotty Creek, NWT, Canada
Potential evaporation at eddy-covariance sites across the globe
Scaling properties reveal regulation of river flows in the Amazon through a “forest reservoir”
Water movement through plant roots – exact solutions of the water flow equation in roots with linear or exponential piecewise hydraulic properties
Large-scale vegetation responses to terrestrial moisture storage changes
Vegetation dynamics and climate seasonality jointly control the interannual catchment water balance in the Loess Plateau under the Budyko framework
Leaf-scale experiments reveal an important omission in the Penman–Monteith equation
The Budyko functions under non-steady-state conditions
Matching the Budyko functions with the complementary evaporation relationship: consequences for the drying power of the air and the Priestley–Taylor coefficient
Hydrological recovery in two large forested watersheds of southeastern China: the importance of watershed properties in determining hydrological responses to reforestation
The socioecohydrology of rainwater harvesting in India: understanding water storage and release dynamics across spatial scales
Nitrate sinks and sources as controls of spatio-temporal water quality dynamics in an agricultural headwater catchment
Impacts of beaver dams on hydrologic and temperature regimes in a mountain stream
Estimation of crop water requirements: extending the one-step approach to dual crop coefficients
Technical Note: On the Matt–Shuttleworth approach to estimate crop water requirements
Horizontal soil water potential heterogeneity: simplifying approaches for crop water dynamics models
Hurricane impacts on a pair of coastal forested watersheds: implications of selective hurricane damage to forest structure and streamflow dynamics
Regional and local patterns in depth to water table, hydrochemistry and peat properties of bogs and their laggs in coastal British Columbia
Impacts of forest changes on hydrology: a case study of large watersheds in the upper reaches of Minjiang River watershed in China
A simple three-dimensional macroscopic root water uptake model based on the hydraulic architecture approach
Training hydrologists to be ecohydrologists and play a leading role in environmental problem solving
Thermodynamic constraints on effective energy and mass transfer and catchment function
Can we predict groundwater discharge from terrestrial ecosystems using existing eco-hydrological concepts?
Macroinvertebrate community responses to a dewatering disturbance gradient in a restored stream
Mechanisms of vegetation uprooting by flow in alluvial non-cohesive sediment
Forest decline caused by high soil water conditions in a permafrost region
Fabien Koch, Philipp Blum, Heide Stein, Andreas Fuchs, Hans Jürgen Hahn, and Kathrin Menberg
Hydrol. Earth Syst. Sci., 28, 4927–4946, https://doi.org/10.5194/hess-28-4927-2024, https://doi.org/10.5194/hess-28-4927-2024, 2024
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In this study, we identify shifts in groundwater fauna due to natural or human impacts over 2 decades. We find no overall temporal or large-scale trends in fauna or abiotic parameters. However, at a local level, six monitoring wells show shifting or fluctuating faunal parameters. Our findings indicate that changes in surface conditions should be assessed in line with hydrochemical parameters to better understand changes in groundwater fauna and to obtain reliable biomonitoring results.
Hongkai Gao, Markus Hrachowitz, Lan Wang-Erlandsson, Fabrizio Fenicia, Qiaojuan Xi, Jianyang Xia, Wei Shao, Ge Sun, and Hubert H. G. Savenije
Hydrol. Earth Syst. Sci., 28, 4477–4499, https://doi.org/10.5194/hess-28-4477-2024, https://doi.org/10.5194/hess-28-4477-2024, 2024
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The concept of the root zone is widely used but lacks a precise definition. Its importance in Earth system science is not well elaborated upon. Here, we clarified its definition with several similar terms to bridge the multi-disciplinary gap. We underscore the key role of the root zone in the Earth system, which links the biosphere, hydrosphere, lithosphere, atmosphere, and anthroposphere. To better represent the root zone, we advocate for a paradigm shift towards ecosystem-centred modelling.
Siwei Chen, Yuxue Guo, Yue-Ping Xu, and Lu Wang
Hydrol. Earth Syst. Sci. Discuss., https://doi.org/10.5194/hess-2024-145, https://doi.org/10.5194/hess-2024-145, 2024
Revised manuscript accepted for HESS
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Our research explores how increased CO2 levels affect water use efficiency in the Yellow River Basin. Using updated climate models, we found that future climate change significantly impacts water efficiency, leading to improved plant resilience against moderate droughts. These findings help predict how ecosystems might adapt to environmental changes, providing essential insights for managing water resources under varying climate conditions.
Xuejin Tan, Bingjun Liu, Xuezhi Tan, Zeqin Huang, and Jianyu Fu
Hydrol. Earth Syst. Sci. Discuss., https://doi.org/10.5194/hess-2024-106, https://doi.org/10.5194/hess-2024-106, 2024
Revised manuscript accepted for HESS
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We assess the spatiotemporal changes in blue and green water scarcity in a anthropogenic highly-impacted watershed and their association with climate change and land use change, using a multi-water-flux validated SWAT model. Observed streamflow, evapotranspiration, and soil moisture are integrated to model calibration, and validation. Results show that both climate change and land use change have decrease blue water and g green water flow, while land use change increase green water flow.
Zongxing Li, Juan Gui, Qiao Cui, Jian Xue, Fa Du, and Lanping Si
Hydrol. Earth Syst. Sci., 28, 719–734, https://doi.org/10.5194/hess-28-719-2024, https://doi.org/10.5194/hess-28-719-2024, 2024
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Precipitation, ground ice, and snow meltwater accounted for approximately 72 %, 20 %, and 8 % of soil water during the early ablation period. Snow is completely melted in the heavy ablation period and the end of the ablation period, and precipitation contributed about 90 % and 94 % of soil water, respectively. These recharges also vary markedly with altitude and vegetation type.
Max Berkelhammer, Gerald F. Page, Frank Zurek, Christopher Still, Mariah S. Carbone, William Talavera, Laura Hildebrand, James Byron, Kyle Inthabandith, Angellica Kucinski, Melissa Carter, Kelsey Foss, Wendy Brown, Rosemary W. H. Carroll, Austin Simonpietri, Marshall Worsham, Ian Breckheimer, Anna Ryken, Reed Maxwell, David Gochis, Mark Raleigh, Eric Small, and Kenneth H. Williams
EGUsphere, https://doi.org/10.5194/egusphere-2023-3063, https://doi.org/10.5194/egusphere-2023-3063, 2024
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Warming in montane systems is affecting the amount of snowmelt inputs. This will affect subalpine forests globally that rely on spring snowmelt to support their water demands. We use a network of sensors across in the Upper Colorado Basin to show that changing spring primarily impacts dense forest stands that have high peak water demands. On the other hand, open forest stands show a higher reliance on summer rain and were minimally sensitive to even historically low snow conditions like 2019.
Licong Dai, Ruiyu Fu, Xiaowei Guo, Yangong Du, Guangmin Cao, Huakun Zhou, and Zhongmin Hu
Hydrol. Earth Syst. Sci., 27, 4247–4256, https://doi.org/10.5194/hess-27-4247-2023, https://doi.org/10.5194/hess-27-4247-2023, 2023
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We found that, in the 0–30 cm soil layer, soil water retention and soil water content in normal Kobresia meadow (NM) were higher than those in biocrust meadow (BM), whereas the 30–40 cm layer's soil water retention and soil water content in NM were lower than those in BM. The topsoil infiltration rate in BM was lower than that in NM. Our findings revealed that the establishment of biocrust did not improve soil water retention and infiltration.
Shaofei Wang, Xiaodong Gao, Min Yang, Gaopeng Huo, Xiaolin Song, Kadambot H. M. Siddique, Pute Wu, and Xining Zhao
Hydrol. Earth Syst. Sci., 27, 123–137, https://doi.org/10.5194/hess-27-123-2023, https://doi.org/10.5194/hess-27-123-2023, 2023
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Water uptake depth of 11-year-old apple trees reached 300 cm in the blossom and young fruit stage and only 100 cm in the fruit swelling stage, while 17-year-old trees always consumed water from 0–320 cm soil layers. Overall, the natural abundance of stable water isotopes method overestimated the contribution of deep soil water, especially in the 320–500 cm soils. Our findings highlight that determining the occurrence of root water uptake in deep soils helps to quantify trees' water use strategy.
Juan Gui, Zongxing Li, Qi Feng, Qiao Cui, and Jian Xue
Hydrol. Earth Syst. Sci., 27, 97–122, https://doi.org/10.5194/hess-27-97-2023, https://doi.org/10.5194/hess-27-97-2023, 2023
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As the transition zone between the Tibetan Plateau and the arid region, the Qilian Mountains are important ecological barriers and source regions of inland rivers in northwest China. In recent decades, drastic changes in the cryosphere have had a significant impact on the quantity and formation process of water resources in the Qilian Mountains. The mountain runoff of the Qilian Mountains mainly comes from the cryosphere belt, which contributes to approximately 80 % runoff.
Remko C. Nijzink and Stanislaus J. Schymanski
Hydrol. Earth Syst. Sci., 26, 6289–6309, https://doi.org/10.5194/hess-26-6289-2022, https://doi.org/10.5194/hess-26-6289-2022, 2022
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Most catchments plot close to the empirical Budyko curve, which allows for estimating the long-term mean annual evaporation and runoff. We found that a model that optimizes vegetation properties in response to changes in precipitation leads it to converge to a single curve. In contrast, models that assume no changes in vegetation start to deviate from a single curve. This implies that vegetation has a stabilizing role, bringing catchments back to equilibrium after changes in climate.
Yakun Tang, Lina Wang, Yongqiang Yu, and Dongxu Lu
Hydrol. Earth Syst. Sci., 26, 4995–5013, https://doi.org/10.5194/hess-26-4995-2022, https://doi.org/10.5194/hess-26-4995-2022, 2022
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Whether rainwater-recharged soil water (RRS) uptake can increase plant transpiration after rainfall pulses requires investigation. Our results indicate a differential response of plant transpiration to RRS uptake. Mixed afforestation enhances these water relationships and decreases soil water source competition in deep soil. Our results suggest that plant species or plantation types that can enhance RRS uptake and reduce water competition should be considered for use in water-limited regions.
Javier de la Casa, Adrià Barbeta, Asun Rodríguez-Uña, Lisa Wingate, Jérôme Ogée, and Teresa E. Gimeno
Hydrol. Earth Syst. Sci., 26, 4125–4146, https://doi.org/10.5194/hess-26-4125-2022, https://doi.org/10.5194/hess-26-4125-2022, 2022
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Recently, studies have been reporting mismatches in the water isotopic composition of plants and soils. In this work, we reviewed worldwide isotopic composition data of field and laboratory studies to see if the mismatch is generalised, and we found it to be true. This contradicts theoretical expectations and may underlie an non-described phenomenon that should be forward investigated and implemented in ecohydrological models to avoid erroneous estimations of water sources used by vegetation.
Amilcare Porporato
Hydrol. Earth Syst. Sci., 26, 355–374, https://doi.org/10.5194/hess-26-355-2022, https://doi.org/10.5194/hess-26-355-2022, 2022
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Applying dimensional analysis to the partitioning of water and soil on terrestrial landscapes reveals their dominant environmental controls. We discuss how the dryness index and the storage index affect the long-term rainfall partitioning, the key nonlinear control of the dryness index in global datasets of weathering rates, and the existence of new macroscopic relations among average variables in landscape evolution statistics with tantalizing analogies with turbulent fluctuations.
Olivia Carpino, Kristine Haynes, Ryan Connon, James Craig, Élise Devoie, and William Quinton
Hydrol. Earth Syst. Sci., 25, 3301–3317, https://doi.org/10.5194/hess-25-3301-2021, https://doi.org/10.5194/hess-25-3301-2021, 2021
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This study demonstrates how climate warming in peatland-dominated regions of discontinuous permafrost is changing the form and function of the landscape. Key insights into the rates and patterns of such changes in the coming decades are provided through careful identification of land cover transitional stages and characterization of the hydrological and energy balance regimes for each stage.
Fabien Koch, Kathrin Menberg, Svenja Schweikert, Cornelia Spengler, Hans Jürgen Hahn, and Philipp Blum
Hydrol. Earth Syst. Sci., 25, 3053–3070, https://doi.org/10.5194/hess-25-3053-2021, https://doi.org/10.5194/hess-25-3053-2021, 2021
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In this study, we address the question of whether groundwater fauna in an urban area is natural or affected in comparison to forested land. We find noticeable differences in the spatial distribution of groundwater species and abiotic parameters. An ecological assessment reveals that conditions in the urban area are mainly not good. Yet, there is no clear spatial pattern in terms of land use and anthropogenic impacts. These are significant findings for conservation and usage of urban groundwater.
James W. Kirchner and Scott T. Allen
Hydrol. Earth Syst. Sci., 24, 17–39, https://doi.org/10.5194/hess-24-17-2020, https://doi.org/10.5194/hess-24-17-2020, 2020
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Perhaps the oldest question in hydrology is
Where does water go when it rains?. Here we present a new way to measure how the terrestrial water cycle partitions precipitation into its two ultimate fates:
green waterthat is evaporated or transpired back to the atmosphere and
blue waterthat is discharged to stream channels. Our analysis may help in gauging the vulnerability of both water resources and terrestrial ecosystems to changes in rainfall patterns.
Yu Liu, Zeng Cui, Ze Huang, Hai-Tao Miao, and Gao-Lin Wu
Hydrol. Earth Syst. Sci., 23, 2481–2490, https://doi.org/10.5194/hess-23-2481-2019, https://doi.org/10.5194/hess-23-2481-2019, 2019
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We focus on the positive effects of litter crusts on soil water holding capacity and water interception capacity compared with biocrusts. Litter crusts can significantly improve sandy water content and organic matter. Water-holding capacity increased with development of litter crusts in the sandy interface. Water infiltration rate is increased by sandy and litter crusts' interface properties. Litter crusts provided a better microhabitat conducive to plant growth in sandy lands.
Adrià Barbeta, Sam P. Jones, Laura Clavé, Lisa Wingate, Teresa E. Gimeno, Bastien Fréjaville, Steve Wohl, and Jérôme Ogée
Hydrol. Earth Syst. Sci., 23, 2129–2146, https://doi.org/10.5194/hess-23-2129-2019, https://doi.org/10.5194/hess-23-2129-2019, 2019
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Plant water sources of a beech riparian forest were monitored using stable isotopes. Isotopic fractionation during root water uptake is usually neglected but may be more common than previously accepted. Xylem water was always more depleted in δ2H than all sources considered, suggesting isotopic discrimination during water uptake or within plant tissues. Thus, the identification and quantification of tree water sources was affected. Still, oxygen isotopes were a good tracer of plant source water.
William Quinton, Aaron Berg, Michael Braverman, Olivia Carpino, Laura Chasmer, Ryan Connon, James Craig, Élise Devoie, Masaki Hayashi, Kristine Haynes, David Olefeldt, Alain Pietroniro, Fereidoun Rezanezhad, Robert Schincariol, and Oliver Sonnentag
Hydrol. Earth Syst. Sci., 23, 2015–2039, https://doi.org/10.5194/hess-23-2015-2019, https://doi.org/10.5194/hess-23-2015-2019, 2019
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This paper synthesizes nearly three decades of eco-hydrological field and modelling studies at Scotty Creek, Northwest Territories, Canada, highlighting the key insights into the major water flux and storage processes operating within and between the major land cover types of this wetland-dominated region of discontinuous permafrost. It also examines the rate and pattern of permafrost-thaw-induced land cover change and how such changes will affect the hydrology and water resources of the region.
Wouter H. Maes, Pierre Gentine, Niko E. C. Verhoest, and Diego G. Miralles
Hydrol. Earth Syst. Sci., 23, 925–948, https://doi.org/10.5194/hess-23-925-2019, https://doi.org/10.5194/hess-23-925-2019, 2019
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Potential evaporation (Ep) is the amount of water an ecosystem would consume if it were not limited by water availability or other stress factors. In this study, we compared several methods to estimate Ep using a global dataset of 107 FLUXNET sites. A simple radiation-driven method calibrated per biome consistently outperformed more complex approaches and makes a suitable tool to investigate the impact of water use and demand, drought severity and biome productivity.
Juan Fernando Salazar, Juan Camilo Villegas, Angela María Rendón, Estiven Rodríguez, Isabel Hoyos, Daniel Mercado-Bettín, and Germán Poveda
Hydrol. Earth Syst. Sci., 22, 1735–1748, https://doi.org/10.5194/hess-22-1735-2018, https://doi.org/10.5194/hess-22-1735-2018, 2018
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River flow regimes are being altered by global change. Understanding the mechanisms behind such alterations is crucial for hydrological prediction. We introduce a novel interpretation of river flow metrics (scaling) that allows any river basin to be classified as regulated or unregulated, and to identify transitions between these states. We propose the
forest reservoirhypothesis to explain how forest loss can force the Amazonian river basins from regulated to unregulated states.
Félicien Meunier, Valentin Couvreur, Xavier Draye, Mohsen Zarebanadkouki, Jan Vanderborght, and Mathieu Javaux
Hydrol. Earth Syst. Sci., 21, 6519–6540, https://doi.org/10.5194/hess-21-6519-2017, https://doi.org/10.5194/hess-21-6519-2017, 2017
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To maintain its yield, a plant needs to transpire water that it acquires from the soil. A deep understanding of the mechanisms that lead to water uptake location and intensity is required to correctly simulate the water transfer in the soil to the atmosphere. This work presents novel and general solutions of the water flow equation in roots with varying hydraulic properties that deeply affect the uptake pattern and the transpiration rate and can be used in ecohydrological models.
Robert L. Andrew, Huade Guan, and Okke Batelaan
Hydrol. Earth Syst. Sci., 21, 4469–4478, https://doi.org/10.5194/hess-21-4469-2017, https://doi.org/10.5194/hess-21-4469-2017, 2017
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In this study we statistically analyse the relationship between vegetation cover and components of total water storage. Splitting water storage into different components allows for a more comprehensive understanding of the temporal response of vegetation to changes in water storage. Generally, vegetation appears to be more sensitive to interannual changes in water storage than to shorter changes, though this varies in different land use types.
Tingting Ning, Zhi Li, and Wenzhao Liu
Hydrol. Earth Syst. Sci., 21, 1515–1526, https://doi.org/10.5194/hess-21-1515-2017, https://doi.org/10.5194/hess-21-1515-2017, 2017
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The relationship between controlling parameters of annual catchment water balance and climate seasonality (S) and vegetation coverage (M) was discussed under the Budyko framework and an empirical equation was further developed so that the contributions from M to actual evapotranspiration (ET) could be determined more accurately. The results showed that the effects of landscape condition changes to ET variation will be estimated with a large error if the impacts of S are ignored.
Stanislaus J. Schymanski and Dani Or
Hydrol. Earth Syst. Sci., 21, 685–706, https://doi.org/10.5194/hess-21-685-2017, https://doi.org/10.5194/hess-21-685-2017, 2017
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Most of the rain falling on land is returned to the atmosphere by plant leaves, which release water vapour (transpire) through tiny pores. To better understand this process, we used artificial leaves in a special wind tunnel and discovered major problems with an established approach (PM equation) widely used to quantify transpiration and its sensitivity to climate change. We present an improved set of equations, consistent with experiments and displaying more realistic climate sensitivity.
Roger Moussa and Jean-Paul Lhomme
Hydrol. Earth Syst. Sci., 20, 4867–4879, https://doi.org/10.5194/hess-20-4867-2016, https://doi.org/10.5194/hess-20-4867-2016, 2016
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A new physically based formulation is proposed to extend the Budyko framework under non-steady-state conditions, taking into account the change in water storage. The new formulation, which introduces an additional parameter, represents a generic framework applicable to any Budyko function at various time steps. It is compared to other formulations from the literature and the analytical solution of Greve et al. (2016) appears to be a particular case.
Jean-Paul Lhomme and Roger Moussa
Hydrol. Earth Syst. Sci., 20, 4857–4865, https://doi.org/10.5194/hess-20-4857-2016, https://doi.org/10.5194/hess-20-4857-2016, 2016
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The Budyko functions are matched with the complementary evaporation relationship. We show that there is a functional dependence between the Budyko functions and the drying power of the air. Examining the case where potential evaporation is calculated by means of a Priestley–Taylor type equation with a varying coefficient, we show that this coefficient should have a specified value as a function of the Budyko shape parameter and the aridity index.
Wenfei Liu, Xiaohua Wei, Qiang Li, Houbao Fan, Honglang Duan, Jianping Wu, Krysta Giles-Hansen, and Hao Zhang
Hydrol. Earth Syst. Sci., 20, 4747–4756, https://doi.org/10.5194/hess-20-4747-2016, https://doi.org/10.5194/hess-20-4747-2016, 2016
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In recent decades, limited research has been conducted to examine the role of watershed properties in hydrological responses in large watersheds. Based on pair-wise comparisons, we conclude that reforestation decreased high flows but increased low flows in the watersheds studied. Hydrological recovery through reforestation is largely dependent on watershed properties when forest change and climate are similar and comparable. This finding has important implications for designing reforestation.
Kimberly J. Van Meter, Michael Steiff, Daniel L. McLaughlin, and Nandita B. Basu
Hydrol. Earth Syst. Sci., 20, 2629–2647, https://doi.org/10.5194/hess-20-2629-2016, https://doi.org/10.5194/hess-20-2629-2016, 2016
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Although village-scale rainwater harvesting (RWH) structures have been used for millennia in India, many of these structures have fallen into disrepair due to increased dependence on groundwater. This dependence has contributed to declines in groundwater resources, and in turn to efforts to revive older RWH systems. In the present study, we use field data to quantify water fluxes in a cascade of irrigation tanks to better our understanding of the impact of RWH systems on the water balance in con
Tobias Schuetz, Chantal Gascuel-Odoux, Patrick Durand, and Markus Weiler
Hydrol. Earth Syst. Sci., 20, 843–857, https://doi.org/10.5194/hess-20-843-2016, https://doi.org/10.5194/hess-20-843-2016, 2016
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We quantify the spatio-temporal impact of distinct nitrate sinks and sources on stream network nitrate dynamics in an agricultural headwater. By applying a data-driven modelling approach, we are able to fully distinguish between mixing and dilution processes, and biogeochemical in-stream removal processes along the stream network. In-stream nitrate removal is estimated by applying a novel transfer coefficient based on energy availability.
M. Majerova, B. T. Neilson, N. M. Schmadel, J. M. Wheaton, and C. J. Snow
Hydrol. Earth Syst. Sci., 19, 3541–3556, https://doi.org/10.5194/hess-19-3541-2015, https://doi.org/10.5194/hess-19-3541-2015, 2015
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This study quantifies the impacts of beaver on hydrologic and temperature regimes, as well as highlights the importance of understanding the spatial and temporal scales of those impacts.
Reach-scale discharge showed shift from losing to gaining. Temperature increased by 0.38°C (3.8%) and mean residence time by 230%. At the sub-reach scale, discharge gains and losses increased in variability. At the beaver dam scale, we observed increase in thermal heterogeneity with warmer and cooler niches.
J. P. Lhomme, N. Boudhina, M. M. Masmoudi, and A. Chehbouni
Hydrol. Earth Syst. Sci., 19, 3287–3299, https://doi.org/10.5194/hess-19-3287-2015, https://doi.org/10.5194/hess-19-3287-2015, 2015
J. P. Lhomme, N. Boudhina, and M. M. Masmoudi
Hydrol. Earth Syst. Sci., 18, 4341–4348, https://doi.org/10.5194/hess-18-4341-2014, https://doi.org/10.5194/hess-18-4341-2014, 2014
V. Couvreur, J. Vanderborght, L. Beff, and M. Javaux
Hydrol. Earth Syst. Sci., 18, 1723–1743, https://doi.org/10.5194/hess-18-1723-2014, https://doi.org/10.5194/hess-18-1723-2014, 2014
A. D. Jayakaran, T. M. Williams, H. Ssegane, D. M. Amatya, B. Song, and C. C. Trettin
Hydrol. Earth Syst. Sci., 18, 1151–1164, https://doi.org/10.5194/hess-18-1151-2014, https://doi.org/10.5194/hess-18-1151-2014, 2014
S. A. Howie and H. J. van Meerveld
Hydrol. Earth Syst. Sci., 17, 3421–3435, https://doi.org/10.5194/hess-17-3421-2013, https://doi.org/10.5194/hess-17-3421-2013, 2013
X. Cui, S. Liu, and X. Wei
Hydrol. Earth Syst. Sci., 16, 4279–4290, https://doi.org/10.5194/hess-16-4279-2012, https://doi.org/10.5194/hess-16-4279-2012, 2012
V. Couvreur, J. Vanderborght, and M. Javaux
Hydrol. Earth Syst. Sci., 16, 2957–2971, https://doi.org/10.5194/hess-16-2957-2012, https://doi.org/10.5194/hess-16-2957-2012, 2012
M. E. McClain, L. Chícharo, N. Fohrer, M. Gaviño Novillo, W. Windhorst, and M. Zalewski
Hydrol. Earth Syst. Sci., 16, 1685–1696, https://doi.org/10.5194/hess-16-1685-2012, https://doi.org/10.5194/hess-16-1685-2012, 2012
C. Rasmussen
Hydrol. Earth Syst. Sci., 16, 725–739, https://doi.org/10.5194/hess-16-725-2012, https://doi.org/10.5194/hess-16-725-2012, 2012
A. P. O'Grady, J. L. Carter, and J. Bruce
Hydrol. Earth Syst. Sci., 15, 3731–3739, https://doi.org/10.5194/hess-15-3731-2011, https://doi.org/10.5194/hess-15-3731-2011, 2011
J. D. Muehlbauer, M. W. Doyle, and E. S. Bernhardt
Hydrol. Earth Syst. Sci., 15, 1771–1783, https://doi.org/10.5194/hess-15-1771-2011, https://doi.org/10.5194/hess-15-1771-2011, 2011
K. Edmaier, P. Burlando, and P. Perona
Hydrol. Earth Syst. Sci., 15, 1615–1627, https://doi.org/10.5194/hess-15-1615-2011, https://doi.org/10.5194/hess-15-1615-2011, 2011
H. Iwasaki, H. Saito, K. Kuwao, T. C. Maximov, and S. Hasegawa
Hydrol. Earth Syst. Sci., 14, 301–307, https://doi.org/10.5194/hess-14-301-2010, https://doi.org/10.5194/hess-14-301-2010, 2010
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Short summary
This study investigates the age and origin of leaf wax n-alkanes from a fluvial sediment–paleosol sequence (FSPS) by compound-class 14C dating. Our results show varying age offsets between the formation and sedimentation of leaf wax n-alkanes from well-developed (paleo)soils and fluvial sediments that are mostly due to their complex origin in such sequences. Thus, dating the leaf wax n-alkanes is an important step for more robust leaf-wax-based paleoenvironmental reconstructions in FSPSs.
This study investigates the age and origin of leaf wax n-alkanes from a fluvial...