To assess the efficiency of the groundwater management of an administrative unit, we propose decomposing the groundwater head changes within an administrative unit into inside and outside contributions by using numerical models. Guantao County of Hebei Province, China, serves as an example to demonstrate the decomposition technique. The groundwater flow model of Guantao was constructed using observed heads as prescribed head boundary conditions. The model was coupled with Hydrus 1-D to calculate the groundwater recharge distribution in time reflecting the delay and damping effects of the soil column on seepage at the surface. The model was calibrated by adjusting parameters such as hydraulic conductivities, recharge infiltration ratios and specific yields. The calibrated parameters are then used in a large model with a boundary at a large distance from Guantao administrative boundary to determine the groundwater head changes due to inside drivers. The differences of the two models on the Guantao boundary serve as the specified head values on the boundary for a small-scale model, which is used to calculate the groundwater head imposed by outside drivers. To eliminate inconsistencies caused by the different types of boundary conditions of large and small models, the groundwater head changes due to inside drivers must be updated. The results indicate that the groundwater head changes in the center and south of Guantao County are influenced equally by both inside and outside contributions, while in the north outside contributions have the stronger impact. On average, 48.5 % of groundwater head changes in the whole of Guantao County is influenced by inside contributions, while 51.5 % is due to outside contributions. The sensitivity analysis shows that the groundwater head changes and their decomposition are much more sensitive to infiltration ratios than to the aquifer parameters. The parameters within Guantao have a certain influence on the net groundwater head changes, while the parameters outside of Guantao only have an influence on the decomposition.

The natural shallow groundwater flow field is usually determined by
infiltration from precipitation and streams, by discharge to streams or
springs and by phreatic evapotranspiration. With the development of human
activities, the natural groundwater levels are modified by land use change,
crop planting and irrigation, groundwater pumping and more. Over the last
few decades, the groundwater resources worldwide have been intensively used
for household, industry and agriculture purposes (Zektser and Everett,
2004). It is estimated that of the approximately 1000 km

To build a groundwater model of an administrative unit is difficult as
usually natural model boundaries do not coincide with political boundaries.
However, we often want to assess the efficiency of groundwater management of an
administrative unit. The groundwater head changes within an administrative
unit are influenced not only by the groundwater head changes induced by
inside drivers, but also by the groundwater head changes induced by outside
drivers. Monitoring groundwater levels within the administrative unit often
cannot directly and faithfully reflect the effects of water management
measures implemented in that unit. In other words, the monitored groundwater
head changes are caused by both inside and outside contributions. Therefore,
we propose to decompose the groundwater head changes over a given time
period within an administrative unit into inside and outside contributions
to assess the efficiency of the unit's management of groundwater resources.
To do so three groundwater models are required:

a model of the administrative unit with the political boundary implemented as a prescribed head boundary using observed heads,

a larger model containing this model, which computes only the propagation of inside changes to the outside and which may extend to physical model boundaries, and

a model of the administrative unit with prescribed heads obtained by subtraction from the previous two models on the political boundary, which is used to determine the groundwater head contributions controlled by outside drivers only.

Numerous studies were carried out in the NCP to understand the large-scale groundwater dynamics employing MODFLOW (Lu et al., 2011; Zhou et al., 2012; Qin et al., 2013). For local management purposes these models are far too crude. But groundwater simulations in smaller administrative units of the NCP have been quite rare up to now. In our study, a groundwater flow model for Guantao is constructed using MODFLOW USG under the pre- and post-processor Visual MODFLOW Flex 2014.1 (VMF) developed by Waterloo Hydrogeologic (Panday et al., 2013).

The objective of this research is to take Guantao as a case study to demonstrate how to decompose the groundwater head changes into inside and outside contributions using numerical models. First the general background and available data are introduced. Then the mathematical method of decomposing the groundwater head changes is described in detail. Following that, a numerical model for the Guantao aquifer system is developed and calibrated under both steady-state and time-varying conditions. Then, both a large-scale model and a small-scale numerical model are developed to separately determine the groundwater head changes due to inside and outside contributions. Finally, the sensitivity of the groundwater head changes and their decomposition with respect to parameters and local management measures are discussed.

The NCP is bordered by the Tai Hang Mountains in the west, the Yellow River
in the south, the Bohai Sea in the east and the Yan Shan Mountains in the
north, and has an area of altogether 140 000 km

Schematic map of the NCP

Guantao has the characteristics of a warm continental monsoon climate: hot
and rainy in summer, and cold and dry in winter with an average annual
precipitation of 532 mm, an average annual potential evaporation of 1516 mm
and an annual mean temperature of 13.4

The Quaternary aquifer of Guantao consists of fine sand layers interbedded
with clay or silt aquitard layers. Vertically it is divided into shallow,
middle and deep layers according to different deposits. Based on previous
studies and the recent hydrogeological investigation by CNACG (2015), the
middle layer mainly consists of clay with an average thickness of around 120 m. It contains saline water with total dissolved solids reaching 10 000 g m

All data required to calibrate a numerical groundwater model for the time between 2003 and 2012 are available. Groundwater heads (provided by GIWP and Handan DWR) are observed at three different frequencies. There are 4 observation points with monthly measurements, 11 observation points with two data records each year and 29 observation points with four measurements each year. Daily precipitation data have been purchased from Guantao Meteorological Bureau (yearly data of precipitation between March and October shown in Fig. 2). Annual channel diversions for irrigation and monthly runoff of the Weiyun River as well as officially recorded annual pumping rates have been collected from the Water Resources Bulletin of Guantao for the period from 2003 to 2012 (Fig. 2). The pumping rate for irrigation is highly dependent on precipitation in the NCP. Pumping rates are generally less in years with higher precipitation. Hence, the data point for 2003 showing a combination of higher precipitation with a larger pumping rate is questionable. The sudden significant decrease in the reported pumping rate after 2006 is also questionable as there were hardly any changes in cropping area, crop types and irrigation methods. Therefore, the pumping rates for these years will be adjusted during manual calibration of the transient numerical model.

Time series of the annual pumping rates in the shallow aquifer shown together with annual precipitation (solid line: reported data; dashed line: values adjusted during calibration).

Groundwater heads in Guantao (

The groundwater heads in Guantao can be determined by the governing equation
below together with a (measured) specified head boundary along the
administrative boundary.

Accordingly, the PDE to determine the groundwater head changes due to inside
drivers is as follows:

The groundwater heads in Guantao caused by outside drivers only can be
obtained by numerically solving the following flow equation:

As mentioned above, to decompose the groundwater heads in Guantao, three
numerical models are used in this research. The first is a small-scale
numerical model within Guantao's administrative boundary to
calculate

The Guantao model boundary is the administrative boundary of Guantao, which is conceptualized as a specified head boundary condition. All available groundwater head observations close to the boundary are made use of by defining the boundary heads by interpolation. The bottom of the aquifer (lower boundary of the model) is defined by the boundary between the shallow aquifer and the aquitard. It is interpolated from the well logs of the hydrological investigation (CNACG, 2015) and is considered impervious.

Precipitation is the main recharge to groundwater in Guantao. Other natural recharge terms include river infiltration of the Weiyun River on the eastern boundary and infiltration from the Weixi channel passing through Guantao from south to north. The Weiyun River infiltration is not explicitly described in the numerical model, but is implicitly considered in the specified head boundary condition. The Weixi channel infiltration is simulated using the river package of MODFLOW. The river level is assumed to be 3 m higher than the deepest river channel bottom level. Guantao is an agricultural county. Apart from the main Weixi channel, there are still numerous smaller sub-channels connected to the Weixi channel to divert and store surface water. Infiltration from these smaller sub-channels is considered part of the areal recharge from irrigation and is simulated as a contribution to the recharge package. This is a common way to deal with the leakage to groundwater from numerous field channels in the irrigated cropland, which can also be found in other similar studies (Rejani et al., 2008; Cao et al., 2013).

Groundwater is the main source of irrigation. This is very common in the NCP (Hu et al., 2010; Zhang et al., 2010). In Guantao, due to lack of surface water, groundwater accounts for over 95 % of total applied irrigation water according to data between 2001 and 2011. Nowadays the traditional conveyance of irrigation water by canals and ditches is replaced by pipe irrigation to increase the conveyance efficiency from wells to the cropland. In the field, ridge irrigation and furrow irrigation are still the primary methods for both groundwater and surface water irrigation. Hence, the irrigation backflow is another important source of groundwater recharge. In the study, the recharge contributions by precipitation, irrigation backflow and canal seepage were added up and implemented in the recharge package. The distribution of agricultural area is obtained from satellite remote sensing images of 2014, by mapping the normalized difference vegetation index (NDVI) in winter and spring (provided by Haijing Wang, hydrosolutions Ltd.). The total agricultural area changes only slightly between 2002 and 2013 according to the statistical year books (GSB, 2002–2013). Hence, the agricultural area is assumed to be constant over the modeled time span.

The depth to groundwater is around 20 m according to the available groundwater head observations, so there is no phreatic evaporation from the aquifer. The discharge is exclusively due to pumping wells extracting groundwater from the aquifer. The water abstraction by pumping is implemented in the well package and the spatial distribution is chosen according to the well locations obtained from the general investigation in 2011 (local communication). The pumping rate of the individual well was determined as a constant fraction of the estimated total annual groundwater abstraction (see Sect. 4.1 below).

The two-dimensional groundwater flow model is constructed using VMF-USG, the
unstructured grid version of USGS-MODFLOW. The spatial discretization
consists of 141 379 cells. The cells are refined around pumping wells. The
top elevation is interpolated from SRTM data downloaded from the website
at

Zonation of hydraulic conductivities and recharge infiltration ratios.

Recharge is the most difficult input to quantify in the simulation. Some
researchers suggest that it is a nonlinear function of the water input at
the surface (Kendy, 2003, 2004; Tan et al., 2014; Min et al., 2015). To simplify
the process, the recharge infiltration ratio (

However, for a transient calculation, the temporal distribution of recharge
also has to be represented adequately to describe its influence on
groundwater-level dynamics correctly. In order to better understand the
time lag of the groundwater-level response to the water input at the ground
surface, the groundwater movement in the unsaturated soil zone was simulated
using Hydrus 1-D (Simunek et al., 2013) in this study. The soil column is
modeled from the ground surface to a depth of 20 m, which is comparable to
the yearly averaged depth to groundwater table in Guantao over the last 10 years. Lu et al. (2011) studied the groundwater recharge at five
representative sites in the NCP (two in the piedmont plain, two in the
alluvial plain and one in the coastal plain) using Hydrus. Guantao is
located in the alluvial plain of the NCP with soils mainly consisting of
silt, clay and silty clay. Since no field sampling, monitoring or
experiments in the soil zone were carried out within the project, the soil
material is assumed to be uniformly distributed in the column. The soil
properties are adopted from the two representative sites in the alluvial
plain cited in Lu et al. (2011). The van Genuchten parameters chosen as
input into Hydrus are the average values from Lu's study (2011):

The groundwater recharge is obtained from the calibrated steady-state model as a percentage of total precipitation plus irrigation, which enters the soil column below the root zone. (All other water applied to the soil is assumed to be consumed by evaporation and plant transpiration.) Monthly inputs are computed according to rainfall and irrigation events with this constant recharge ratio. Due to the large depth to groundwater of 20 m and more the water input is delayed and attenuated. The final temporal distribution of the flux at the groundwater table is calculated in the Hydrus simulation. The upper boundary of the column is implemented as an atmospheric boundary to the surface layer, while a free drainage condition is implemented at the lower boundary. The initial distribution of water content is obtained by running the simulation periodically for 10 years to get a relatively steady distribution.

The aim of the model calibration is to minimize the residuals between the
observed and computed head values by adjusting model parameters. We start
out with a steady-state model. The average behavior in the period from 2003
to 2011 was used as a quasi-steady state. This is feasible, as the average
head over all observations at the end of 2002 is almost identical to that at
the end of 2011. That means that on average, abstractions must have been
balanced by recharge over that period. All inputs required in this case are
average data sets between 2003 and 2011. The steady-state model calibration
was accomplished using the automated parameter estimation code (PEST)
(Doherty, 2003). The transient flow model between 2003 and 2012 is
calibrated manually, as only the specific yield values have to be adjusted.
The groundwater flow field obtained from the steady-state model is used as
the initial condition of the transient model. The transient model time span
was divided into monthly stress periods. There are in total 120 stress
periods. The whole calibration process is as follows. Initially, the
officially reported (but estimated) time series of the pumping rate and
inferred recharge ratios are input into Hydrus 1-D to obtain the average
groundwater recharge between 2003 and 2011. Hydrus 1-D is run for each
township using different seepage water input values according to the
collected data. Then the parameter estimation model PEST is applied to
calibrate parameters (

After model calibration, several statistical indices were used to assess the
results of the numerical model. The correlation coefficient

The automatically calibrated values of hydraulic conductivities and recharge infiltration ratios and their respective sensitivities to observed heads.

The zonal values of hydraulic conductivities and recharge infiltration
ratios obtained from PEST in the calibration of the steady-state model are
presented in Table 1. The values of hydraulic conductivities indicate a
decreasing trend from south to north. The relatively less permeable zone
between

The sensitivities of different parameters to observed heads are shown in
Table 1. The parameter (composite) sensitivities are automatically computed
by PEST and saved in the file *.sen. They are calculated according to the
weighted Jacobian matrix and the number of observations (Doherty, 2003). The
table indicates that compared to hydraulic conductivities, the recharge
infiltration ratios have a much larger influence on groundwater heads. The
sensitivity of hydraulic conductivity is higher in the south than in the
north. The most sensitive recharge infiltration ratio is found in the east.
The correlations between different parameters are presented in Table 2.
Correlation coefficients with a modulus above 0.5 indicate that there is a
non-negligible correlation among the respective parameters. The highest
(anti-)correlation coefficient between two zonal hydraulic conductivities
is

The recharge fluxes at different soil depths for one of the eight townships are shown in Fig. 4. They capture the important characteristics of the soil water flux at different depths. The response time becomes longer with increasing depth to groundwater, while the peak flux becomes smaller with a more even distribution over the year. Similar results can be observed in other areas of the NCP (Li et al., 2017; Min et al., 2017). Although the water input on the soil surface is quite different from year to year, few peaks are observed when the soil depth is larger than 10 m, due to damping.

Correlation coefficients among different parameters.

Calculated monthly recharge flux at different soil depths.

The peaks vanish more quickly with increasing soil depth in dry years than in wet years. Despite the averaging, the bottom flux distribution over a year is different from year to year. Even at 20 m depth the biggest difference between the highest and lowest fluxes is still around 30 % of the lowest flux. The groundwater recharge is a complex nonlinear process which mixes all the irrigation and precipitation events occurring at different times. Through the analysis of results from Hydrus, it is obvious that the best way to accurately describe the groundwater recharge in the groundwater model is to couple the model of the unsaturated zone with the groundwater model. The recharge fluxes for other townships demonstrate a similar distribution.

Calculated and observed monthly time series of groundwater heads at four available long-term observation wells.

The specific yield has the same zonation as the hydraulic conductivity. Four
zones of specific yield, denoted by

Discretization map of the large model.

Parameter distributions map for the NCP (modified based on figures in the literature; Liu et al., 2011).

The goodness of fit between modeled and observed groundwater heads is
presented in Fig. 5. Some computed heads underestimate observations and
others overestimate observations. There is no general bias. The seasonal
pattern of groundwater-level dynamics is reproduced. The groundwater level
starts to decrease from March due to irrigation and reaches its lowest value
in June or July. From June or July on, groundwater levels start to recover
and increase in response to termination of pumping and the delayed recharge
by precipitation and irrigation. The large deviations between observations
and computation during the first year are caused by inconsistent initial
groundwater heads, which are “forgotten” after about 1 year. Remember that
the steady-state solution taken as the initial head distribution corresponds
more to the average situation over the 9-year period than to the initial
distribution in 2003. The

Groundwater contour map of the steady state (in m a.s.l.).

Sources and sinks in the large flow model are conceptualized similarly to the Guantao model. The infiltration from precipitation and infiltration from applied irrigation water were calculated with Hydrus 1-D and combined in the groundwater recharge package. The Weixi channel infiltration is simulated as a defined flux boundary instead of using the river package. The infiltration flux is extracted from the Guantao model and then assigned to corresponding cells in the large model. The groundwater discharge from pumping wells is simulated in the well package. An adequate zero-flux boundary of the large flow model is defined by testing the sensitivity of the heads at the boundary location to sources and sinks in Guantao. The boundary is sufficiently far away from Guantao if heads induced by Guantao sources and sinks are close to zero. As a result, the following boundary was chosen: in the west the model is bounded by the mountains, while it is bounded by the Yellow River in the east. These boundaries coincide with the natural boundaries of the NCP. The northeast and southwest are chosen approximately parallel to groundwater contour lines (Fig. 6a), which are sufficiently far away to exclude any influence of Guantao sources and sinks. As only the effect of Guantao drivers is of interest in the large model, all sources and sinks outside of Guantao are set equal to zero.

To solve the large model, its parameter distributions are required. The absolute values of parameters outside of Guantao in the large model are not decisive in the study; only the parameter values close to the Guantao boundary are important. The hydraulic conductivity and specific yield within Guantao have the same values as the calibrated parameters from the Guantao flow model, while the model parameters outside of Guantao are taken from the literature (Liu et al., 2011). The parameter distributions used in the large model are shown in Fig. 7. The sensitivity of the results with respect to the large model's parameters will be explored later. The large groundwater flow model is also constructed using VMF-USG. The modeled area is discretized into 144 829 cells horizontally (Fig. 6). The transmissivity is calculated by multiplying the hydraulic conductivities by the aquifer thickness obtained from the Guantao model in each time step, which means that the transmissivity is constant in each time step but is updated from time step to time step to take into account the changing saturated aquifer thickness. The aquifer thickness outside of Guantao is assumed equal to the average aquifer thickness of the Guantao area. The initial condition is set to zero, which is based on the assumption that the inside drivers of Guantao are in a quasi-steady state. This is consistent with the Guantao flow model, which uses the results from the steady-state model as the initial condition in the transient model.

The model for outside contributions is a small-scale model with the Guantao
administrative boundary as the model boundary. The model structure and
parameters are defined in the same way as in the Guantao flow model. Since
this model is used to determine the groundwater head within Guantao caused
by outside drivers, the source and sink terms inside are set to zero. The
transmissivity used in the model is defined in the same way as in the large
model. The specified head values on the Guantao border are obtained by
subtracting the head changes determined by the large flow model from the
measured heads on the boundary. Since the initial heads for the large model
are zero everywhere, the initial heads for the

The groundwater contour map calculated from the steady-state model is
presented in Fig. 8. Two groundwater depression cones have formed in
Guantao, which have a dominant influence on the groundwater flow direction,
with head gradients from the outside towards the centers of the depression
cones. The large-scale regional groundwater flow is directed across the NCP
from southwest to northeast. Due to over-pumping, the groundwater level has
been declining continuously since the 1960s (Cao et al., 2013). The
intensive local pumping caused the development of numerous depression cones
in the NCP. Analysis of past data shows that the depression cone in Guantao
formed in the early 2000s (Zheng et al., 2010; Shao et al., 2013; Cao et
al., 2013). The groundwater flow characteristics are consistent with the
conclusions from former studies. Groundwater-level gradients are steeper in
the east than in the west, which is caused by the higher observed head
values on the eastern boundary, especially in its southeastern and
northeastern sections. The groundwater recharge from precipitation and
irrigation amounts to 141 000 m

Annual water budget for the period 2003–2012.

The groundwater balance of the transient model is presented in Fig. 9. The
boundary inflow and main channel infiltration are not shown in the figure
because they occupy only a small part of the total groundwater recharge. The
infiltration from precipitation and irrigation fluctuates gently with time
due to the delayed and damped groundwater recharge from precipitation and
irrigation backflow through the long soil column as discussed in Sect.
3.2.1. The pumping rate fluctuates strongly in the first 6 years, while
after that its variability decreases. This is due to the temporal behavior
of precipitation, which directly (and without delay) influences the
groundwater withdrawals for irrigation in summer (Fig. 2). The aquifer
storage increases when groundwater recharge exceeds groundwater withdrawals.
This is the case in 2003, where groundwater storage recovers by

The spatial distribution of the groundwater head and its
decomposition in Guantao at the final time step.

After running the three corresponding numerical models, the spatial
distribution of the groundwater level and its decomposition at the final
time step are presented in Fig. 10. The large light green area in Fig. 10a
with

The groundwater head in Guantao and its decomposition obtained from
numerical models are supposed to satisfy Eq. (1). The difference between the

The groundwater head in the Guantao flow model can be decomposed at any grid
point and at any time. The time series of groundwater heads and their
decomposition at three chosen locations are shown in Fig. 11 (two are
located within Guantao and one is on the boundary). The black solid line
refers to

Time series of groundwater heads in Guantao at three selected locations and their decomposition.

The contour color map of groundwater head changes between the last and
first time steps and its decomposition into inside and outside contributions
are shown in Fig. 12. Figure 12a shows that the groundwater heads
decrease in the south and increase in the north, with

Spatial distribution of changes in groundwater head over the modeled time span and its decomposition.

To explore the groundwater head change and its decomposition in detail,
three specific locations are chosen (Fig. 11). The groundwater head change
in the north of Guantao County increases by 0.9 m over the modeled time
span, resulting from a decrease in

The sensitivity of the model to parameter changes is analyzed to test its
robustness. The parameters, hydraulic conductivities and specific yields
are perturbed by an increase of 50 % in the individual runs, while the
recharge infiltration ratios are perturbed by an increase of 20 %,
respectively. (Parameters include four hydraulic conductivity values

The model sensitivity to parameters is expressed by the normalized composite
sensitivity (

The normalized sensitivities of the Guantao head change (

The normalized sensitivity of head change and contributions to parameters and recharge ratios.

Similar simulations are also carried out regarding the Guantao pumping
rates. In a sensitivity test the pumping rate is increased by 20 %. The
procedures to guarantee consistency are similar to those used for changing
the recharge infiltration ratios (see Sect. 4.4). The spatial distributions
of groundwater head changes and their decomposition with the perturbed
pumping rate are shown in Fig. 14. The differences in groundwater head
changes range from

Two specific locations (one in the south and the other in the north) are
chosen to analyze the influences from inside and outside contributions on
the groundwater head changes. The

Spatial distribution of groundwater head change over the modeled time span and its decomposition: influence of decreased pumping rate.

To explore the impact of the boundary conditions on the groundwater head
change and its decomposition, the Guantao model is run with specified heads
on the boundary increased by 2 m uniformly. The differences between the
models with and without changing the values of the boundary heads are shown
in Fig. 15. Positive values indicate an increasing trend in the component
compared to the results without increased specified head values. Since there
are no changes in sources and sinks in Guantao, the difference in

Differences between the model runs with and without increased specified heads on the boundary.

This study demonstrates how to decompose the groundwater head changes within
a political boundary into inside and outside contributions using numerical
models. The groundwater head in Guantao was calculated using the Guantao
flow model. The groundwater head changes on the Guantao boundary caused by
inside drivers were computed in a large model with a boundary far from the
Guantao administrative boundary. The difference between values on the
Guantao boundary from the two models is assigned as a specified head boundary
condition for the

The steady-state model of Guantao was used to calibrate hydraulic
conductivities and recharge infiltration ratios using data averaged over the
9-year time interval from 2003 to 2011. All hydraulic conductivities and
recharge ratios are sensitive to head observations, with recharge
infiltration ratios having higher sensitivities than hydraulic
conductivities. The identified recharge infiltration ratios are correlated
with each other, with correlation coefficients around

Based on numerical models discussed in the study, the groundwater head in
Guantao at any time and at any point can be decomposed into the groundwater
head changes determined by inside drivers and the groundwater head
determined by outside drivers. The groundwater head change over the whole
modeled time span can correspondingly be decomposed. The groundwater head
in Guantao decreased by

The sensitivity of groundwater head change and its decomposition to various
model parameters was analyzed by perturbing parameters by 50 % and 20 %.
The results show that model outputs are sensitive to hydraulic
conductivities, specific yields and recharge infiltration ratios within
Guantao itself. Parameters outside of Guantao have an influence on the large
model and the

All sources of data are mentioned in the paper. Due to the local authorities' data policy, all data can be accessed by personal request only.

NL conducted the model simulations. NL and WK performed the analysis and wrote the manuscript. HL and WL contributed to the data, analysis of results and model setup. FC contributed to the data and model setup.

The authors declare that they have no conflict of interest.

This research was supported financially by the Swiss Agency for Development and Cooperation (SDC) under the project “Rehabilitation and management strategy for over-pumped aquifers under a changing climate”. We thank Junfang Gu and Hongliang Liu (Handan Department of Water Resources) and Huaixian Yao, Fei Gao and Guangchao Li (Guantao Department of Water Resources) for the tremendous effort they put into our data collection.

This paper was edited by Bill X. Hu and reviewed by two anonymous referees.