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  <front>
    <journal-meta>
<journal-id journal-id-type="publisher">HESS</journal-id>
<journal-title-group>
<journal-title>Hydrology and Earth System Sciences</journal-title>
<abbrev-journal-title abbrev-type="publisher">HESS</abbrev-journal-title>
<abbrev-journal-title abbrev-type="nlm-ta">Hydrol. Earth Syst. Sci.</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1607-7938</issn>
<publisher><publisher-name>Copernicus Publications</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>

    <article-meta>
      <article-id pub-id-type="doi">10.5194/hess-21-779-2017</article-id><title-group><article-title><?xmltex \hack{\vspace*{5mm}}?> The residence time of water in the atmosphere revisited</article-title>
      </title-group><?xmltex \runningtitle{The residence time of water in the atmosphere revisited}?><?xmltex \runningauthor{Ruud~J.~van~der~Ent and Obbe~A.~Tuinenburg}?>
      <contrib-group>
        <contrib contrib-type="author" corresp="yes" rid="aff1">
          <name><surname>van der Ent</surname><given-names>Ruud J.</given-names></name>
          <email>r.j.vanderent@uu.nl</email>
        <ext-link>https://orcid.org/0000-0001-5450-4333</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2">
          <name><surname>Tuinenburg</surname><given-names>Obbe A.</given-names></name>
          
        <ext-link>https://orcid.org/0000-0001-6895-0094</ext-link></contrib>
        <aff id="aff1"><label>1</label><institution>Department of Physical Geography, Faculty of Geosciences, Utrecht University, Utrecht, the Netherlands</institution>
        </aff>
        <aff id="aff2"><label>2</label><institution>Department of Environmental Sciences, Copernicus Institute for Sustainable development, Utrecht University, <?xmltex \hack{\newline}?> Utrecht, the Netherlands</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Ruud J. van der Ent (r.j.vanderent@uu.nl)</corresp></author-notes><pub-date><day>8</day><month>February</month><year>2017</year></pub-date>
      
      <volume>21</volume>
      <issue>2</issue>
      <fpage>779</fpage><lpage>790</lpage>
      <history>
        <date date-type="received"><day>22</day><month>August</month><year>2016</year></date>
           <date date-type="rev-request"><day>1</day><month>September</month><year>2016</year></date>
           <date date-type="rev-recd"><day>17</day><month>January</month><year>2017</year></date>
           <date date-type="accepted"><day>19</day><month>January</month><year>2017</year></date>
      </history>
      <permissions>
<license license-type="open-access">
<license-p>This work is licensed under a Creative Commons Attribution 3.0 Unported License. To view a copy of this license, visit <ext-link ext-link-type="uri" xlink:href="http://creativecommons.org/licenses/by/3.0/">http://creativecommons.org/licenses/by/3.0/</ext-link></license-p>
</license>
</permissions><self-uri xlink:href="https://hess.copernicus.org/articles/21/779/2017/hess-21-779-2017.html">This article is available from https://hess.copernicus.org/articles/21/779/2017/hess-21-779-2017.html</self-uri>
<self-uri xlink:href="https://hess.copernicus.org/articles/21/779/2017/hess-21-779-2017.pdf">The full text article is available as a PDF file from https://hess.copernicus.org/articles/21/779/2017/hess-21-779-2017.pdf</self-uri>


      <abstract>
    <p>This paper revisits the knowledge on the residence time of water in the
atmosphere. Based on state-of-the-art data of the hydrological cycle we
derive a global average residence time of 8.9 <inline-formula><mml:math id="M1" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4 days (uncertainty
given as 1 standard deviation). We use two different atmospheric moisture
tracking models (WAM-2layers and 3D-T) to obtain atmospheric residence time
characteristics in time and space. The tracking models estimate the global
average residence time to be around 8.5 days based on ERA-Interim data. We
conclude that the statement of a recent study that the global average
residence time of water in the atmosphere is 4–5 days, is not correct. We
derive spatial maps of residence time, attributed to evaporation and
precipitation, and age of atmospheric water, showing that there are different
ways of looking at temporal characteristics of atmospheric water. Longer
evaporation residence times often indicate larger distances towards areas of
high precipitation. From our analysis we find that the residence time over
the ocean is about 2 days less than over land. It can be seen that in
winter, the age of atmospheric moisture tends to be much lower than in
summer. In the Northern Hemisphere, due to the contrast in ocean-to-land
temperature and associated evaporation rates, the age of atmospheric moisture
increases following atmospheric moisture flow inland in winter, and decreases
in summer. Looking at the probability density functions of atmospheric
residence time for precipitation and evaporation, we find long-tailed
distributions with the median around 5 days. Overall, our research confirms
the 8–10-day traditional estimate for the global mean residence time of
atmospheric water, and our research contributes to a more complete view of
the characteristics of the turnover of water in the atmosphere in time and
space.</p>
  </abstract>
    </article-meta>
  </front>
<body>
      

      <?xmltex \hack{\newpage}?>
<sec id="Ch1.S1" sec-type="intro">
  <title>Introduction</title>
      <p>The time it takes before evaporated water from land and oceans is returned to
the land surface as precipitation is a fundamental characteristic of the
Earth's hydrological cycle. This atmospheric residence time of moisture is
not often discussed in the scientific research literature. The global average
residence time of atmospheric moisture is mostly seen as non-controversial
knowledge in textbooks <xref ref-type="bibr" rid="bib1.bibx4 bib1.bibx12 bib1.bibx14 bib1.bibx43" id="paren.1"><named-content content-type="pre">e.g.,</named-content></xref>, general water
literature <xref ref-type="bibr" rid="bib1.bibx1 bib1.bibx22" id="paren.2"><named-content content-type="pre">e.g.,</named-content></xref> and educational web pages
<xref ref-type="bibr" rid="bib1.bibx34" id="paren.3"><named-content content-type="pre">e.g.,</named-content></xref>. All of these examples estimate the global average
residence time of atmospheric moisture based on the size of the atmospheric
reservoir divided by the incoming or outgoing flux and as such arrive at
estimates in the range of 0.022–0.027 years or 8–10 days.</p>
      <p>While the global average residence time is a simple estimate, spatial and
temporal pictures of residence times are more difficult to provide. Local
depletion times, given by <inline-formula><mml:math id="M2" display="inline"><mml:mrow><mml:mi>W</mml:mi><mml:mo>/</mml:mo><mml:mi>P</mml:mi></mml:mrow></mml:math></inline-formula>, and local restoration times, given by <inline-formula><mml:math id="M3" display="inline"><mml:mrow><mml:mi>W</mml:mi><mml:mo>/</mml:mo><mml:mi>E</mml:mi></mml:mrow></mml:math></inline-formula>
(where <inline-formula><mml:math id="M4" display="inline"><mml:mi>W</mml:mi></mml:math></inline-formula> is water in the local atmospheric column, <inline-formula><mml:math id="M5" display="inline"><mml:mi>P</mml:mi></mml:math></inline-formula> is precipitation and
<inline-formula><mml:math id="M6" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula> is evaporation), were computed near-globally by <xref ref-type="bibr" rid="bib1.bibx28" id="text.4"/>
and <xref ref-type="bibr" rid="bib1.bibx37" id="text.5"/>. When horizontal moisture transport is small
compared to precipitation and evaporation they provide a proxy for the
residence time. However, it is safer to interpret them as local timescales of
atmospheric moisture recycling <xref ref-type="bibr" rid="bib1.bibx37" id="paren.6"/>. <xref ref-type="bibr" rid="bib1.bibx28" id="text.7"/>
found a global average residence time of atmospheric moisture of 8.9 days
based on evaporation and 9.1 days based on precipitation, and attributed this
difference to the input data having a non-closure of the global water
balance. On the other hand, global spatial average local depletion times and
restoration times were found to be 8.1 and 8.5 days, respectively. The
difference with the global moisture-weighted values was explained by the
heterogeneous distribution of evaporation and precipitation over the Earth
and their spatial correlation with atmospheric moisture.</p>
      <p>Moisture tracking models also allow for the estimation of atmospheric
moisture residence time. A semi-Lagrangian method of passive water vapor
tracers in a general circulation model was used to perform a special
experiment in which all atmospheric water was tagged, after which it was
evaluated how quickly the tagged water rains out
<xref ref-type="bibr" rid="bib1.bibx2 bib1.bibx3" id="paren.8"/>. To clarify, in this experiment the
atmosphere was replenished by evaporation, but this water was not tagged. The
outcome of this analysis was a global average residence time of 8.5 days in
May <xref ref-type="bibr" rid="bib1.bibx2" id="paren.9"/> and 9.2 days in an undefined time period
<xref ref-type="bibr" rid="bib1.bibx3" id="paren.10"/>, respectively. The same types of experiments were
performed by <xref ref-type="bibr" rid="bib1.bibx45" id="text.11"/> with an offline one-layer Eulerian
moisture tracking model using the global GAME reanalysis data. They found a
global mean residence time of between 7.3 days (April) and 9.2 days (August).</p>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T1" specific-use="star"><caption><p>Non-exhaustive overview of (near-)global residence time estimates
for water in the atmosphere in previous studies. Note that the estimates from
this study are shown in Fig. 1.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.97}[.97]?><oasis:tgroup cols="4">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:colspec colnum="3" colname="col3" align="right"/>
     <oasis:colspec colnum="4" colname="col4" align="left"/>
     <oasis:thead>
       <oasis:row>

         <oasis:entry colname="col1">Study</oasis:entry>

         <oasis:entry colname="col2">Physical quantity estimated</oasis:entry>

         <oasis:entry colname="col3">Value</oasis:entry>

         <oasis:entry colname="col4">Method</oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col1"/>

         <oasis:entry colname="col2"/>

         <oasis:entry colname="col3">(days)</oasis:entry>

         <oasis:entry colname="col4"/>

       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>

         <oasis:entry colname="col1"><xref ref-type="bibr" rid="bib1.bibx4" id="text.12"/></oasis:entry>

         <oasis:entry colname="col2">Residence time (global average)</oasis:entry>

         <oasis:entry colname="col3">8.2</oasis:entry>

         <oasis:entry colname="col4">Global water balance</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><xref ref-type="bibr" rid="bib1.bibx14" id="text.13"/></oasis:entry>

         <oasis:entry colname="col2">Residence time (global average)</oasis:entry>

         <oasis:entry colname="col3">9.9</oasis:entry>

         <oasis:entry colname="col4">Global water balance</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><xref ref-type="bibr" rid="bib1.bibx28" id="text.14"/></oasis:entry>

         <oasis:entry colname="col2">Residence time (global average)</oasis:entry>

         <oasis:entry colname="col3">9.1</oasis:entry>

         <oasis:entry colname="col4">Global water balance (<inline-formula><mml:math id="M7" display="inline"><mml:mi>P</mml:mi></mml:math></inline-formula>-based)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><xref ref-type="bibr" rid="bib1.bibx28" id="text.15"/></oasis:entry>

         <oasis:entry colname="col2">Residence time (global average)</oasis:entry>

         <oasis:entry colname="col3">8.9</oasis:entry>

         <oasis:entry colname="col4">Global water balance (<inline-formula><mml:math id="M8" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula>-based)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><xref ref-type="bibr" rid="bib1.bibx28" id="text.16"/></oasis:entry>

         <oasis:entry colname="col2">Depletion time (spatial global average)</oasis:entry>

         <oasis:entry colname="col3">8.1</oasis:entry>

         <oasis:entry colname="col4">Local water balance (<inline-formula><mml:math id="M9" display="inline"><mml:mi>P</mml:mi></mml:math></inline-formula>-based)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><xref ref-type="bibr" rid="bib1.bibx28" id="text.17"/></oasis:entry>

         <oasis:entry colname="col2">Restoration time (spatial global average)</oasis:entry>

         <oasis:entry colname="col3">8.5</oasis:entry>

         <oasis:entry colname="col4">Local water balance (<inline-formula><mml:math id="M10" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula>-based)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><xref ref-type="bibr" rid="bib1.bibx22" id="text.18"/></oasis:entry>

         <oasis:entry colname="col2">Residence time (global average)</oasis:entry>

         <oasis:entry colname="col3">8.6</oasis:entry>

         <oasis:entry colname="col4">Global water balance</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><xref ref-type="bibr" rid="bib1.bibx43" id="text.19"/></oasis:entry>

         <oasis:entry colname="col2">Residence time (global average)</oasis:entry>

         <oasis:entry colname="col3">9.5</oasis:entry>

         <oasis:entry colname="col4">Global water balance</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1" morerows="1"><xref ref-type="bibr" rid="bib1.bibx2" id="text.20"/></oasis:entry>

         <oasis:entry colname="col2" morerows="1">Residence time (global average)</oasis:entry>

         <oasis:entry colname="col3" morerows="1">8.5</oasis:entry>

         <oasis:entry colname="col4">Online tracking method: tagged water</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col4">depletion experiment (during May)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1" morerows="1"><xref ref-type="bibr" rid="bib1.bibx3" id="text.21"/></oasis:entry>

         <oasis:entry colname="col2" morerows="1">Residence time (global average)</oasis:entry>

         <oasis:entry colname="col3" morerows="1">9.2</oasis:entry>

         <oasis:entry colname="col4">Online tracking method: tagged water</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col4">depletion experiment (period not specified)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1" morerows="1"><xref ref-type="bibr" rid="bib1.bibx45" id="text.22"/></oasis:entry>

         <oasis:entry colname="col2" morerows="1">Residence time (global average)</oasis:entry>

         <oasis:entry colname="col3" morerows="1">7.3</oasis:entry>

         <oasis:entry colname="col4">Offline tracking method: tagged water</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col4">depletion experiment (April)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1" morerows="1"><xref ref-type="bibr" rid="bib1.bibx45" id="text.23"/></oasis:entry>

         <oasis:entry colname="col2" morerows="1">Residence time (global average)</oasis:entry>

         <oasis:entry colname="col3" morerows="1">9.2</oasis:entry>

         <oasis:entry colname="col4">Offline tracking method: tagged water</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col4">depletion experiment (August)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><xref ref-type="bibr" rid="bib1.bibx12" id="text.24"/></oasis:entry>

         <oasis:entry colname="col2">Residence time (global average)</oasis:entry>

         <oasis:entry colname="col3">10</oasis:entry>

         <oasis:entry colname="col4">Global water balance</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><xref ref-type="bibr" rid="bib1.bibx34" id="text.25"/></oasis:entry>

         <oasis:entry colname="col2">Residence time (global average)</oasis:entry>

         <oasis:entry colname="col3">9</oasis:entry>

         <oasis:entry colname="col4">Global water balance</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><xref ref-type="bibr" rid="bib1.bibx1" id="text.26"/></oasis:entry>

         <oasis:entry colname="col2">Residence time (global average)</oasis:entry>

         <oasis:entry colname="col3">9.5</oasis:entry>

         <oasis:entry colname="col4">Global water balance</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><xref ref-type="bibr" rid="bib1.bibx41" id="text.27"/></oasis:entry>

         <oasis:entry colname="col2">Residence time (land <inline-formula><mml:math id="M11" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula> only)</oasis:entry>

         <oasis:entry colname="col3">8.7</oasis:entry>

         <oasis:entry colname="col4">Offline tracking method: Eulerian age accounting</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><xref ref-type="bibr" rid="bib1.bibx41" id="text.28"/></oasis:entry>

         <oasis:entry colname="col2">Residence time (land <inline-formula><mml:math id="M12" display="inline"><mml:mi>P</mml:mi></mml:math></inline-formula> only)</oasis:entry>

         <oasis:entry colname="col3">9.7</oasis:entry>

         <oasis:entry colname="col4">Offline tracking method: Eulerian age accounting</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><xref ref-type="bibr" rid="bib1.bibx41" id="text.29"/></oasis:entry>

         <oasis:entry colname="col2">Residence time (<inline-formula><mml:math id="M13" display="inline"><mml:mi>P</mml:mi></mml:math></inline-formula> of land origin only)</oasis:entry>

         <oasis:entry colname="col3">6.4</oasis:entry>

         <oasis:entry colname="col4">Offline tracking method: Eulerian age accounting</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><xref ref-type="bibr" rid="bib1.bibx17" id="text.30"/></oasis:entry>

         <oasis:entry colname="col2">Residence time (spatial global average)</oasis:entry>

         <oasis:entry colname="col3">8.3</oasis:entry>

         <oasis:entry colname="col4">Local Eulerian method with transport</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1" morerows="1"><xref ref-type="bibr" rid="bib1.bibx17" id="text.31"/></oasis:entry>

         <oasis:entry colname="col2" morerows="1">Residence time (global average)</oasis:entry>

         <oasis:entry colname="col3" morerows="1">3.9</oasis:entry>

         <oasis:entry colname="col4">Offline tracking method: Lagrangian trajectories</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col4">(15 days, for which all figures are presented)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><xref ref-type="bibr" rid="bib1.bibx17" id="text.32"/></oasis:entry>

         <oasis:entry colname="col2">Residence time (global average)</oasis:entry>

         <oasis:entry colname="col3">4.4</oasis:entry>

         <oasis:entry colname="col4">Offline tracking method: trajectories (20 days)</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1" morerows="1"><xref ref-type="bibr" rid="bib1.bibx17" id="text.33"/></oasis:entry>

         <oasis:entry colname="col2" morerows="1">Residence time (global average)</oasis:entry>

         <oasis:entry colname="col3" morerows="1">4–5</oasis:entry>

         <oasis:entry colname="col4">Expert judgment based on tracking results and</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col4">assumptions</oasis:entry>

       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table></table-wrap>

      <p>The global experiments of <xref ref-type="bibr" rid="bib1.bibx3" id="text.34"/> and <xref ref-type="bibr" rid="bib1.bibx45" id="text.35"/>
also suggest that the time it takes before atmospheric water rains out has a
negative exponential distribution, which belongs to a Poisson process
<xref ref-type="bibr" rid="bib1.bibx10" id="paren.36"><named-content content-type="pre">e.g.,</named-content></xref>. The median residence time can be estimated
from the graphs provided by <xref ref-type="bibr" rid="bib1.bibx3" id="text.37"/> and <xref ref-type="bibr" rid="bib1.bibx45" id="text.38"/>
as around 6 days. On a more local scale with a pure Lagrangian moisture
tracking method applied in India, <xref ref-type="bibr" rid="bib1.bibx33" id="text.39"/> showed probability
density functions of the time that evaporated water remains in the atmosphere
before it precipitates again. They found that evaporated water has the
highest probability of staying in the atmosphere for around 5 days, but that
there is a long tail of the probability distribution as many water particles
still reside in the atmosphere more than 25 days after evaporation,
suggesting the mean to be much higher than the median.</p>
      <p>In a near-global study <xref ref-type="bibr" rid="bib1.bibx41" id="text.40"/> extended
Eulerian moisture tracking model WAM-2layers to calculate both the amount and age of
tracked water. Forcing their model with precipitation, wind and humidity from
ERA-Interim (ERA-I) <xref ref-type="bibr" rid="bib1.bibx5" id="paren.41"/>, and evaporation from global
hydrological model STEAM <xref ref-type="bibr" rid="bib1.bibx42" id="paren.42"/>, they computed atmospheric
residence times over land. As such, they found that the residence time of
land precipitation is 9.7 days and that of precipitation recycled over land
is 6.4 days. For evaporation they found a residence time of 8.7 days, with
fast evaporation processes (interception, soil and open water evaporation)
having a residence time of 8.1 days vs. a residence time of 9.1 days for
transpiration. In addition to these averages, they also showed spatial maps
of residence times, but these refer to the fraction that recycles only, which
is relatively fast compared to the average residence times. South America
popped up as the continent with the lowest atmospheric residence times, which
were shown to be around 4 days for moisture recycling over land. As explained
above, residence times of atmospheric moisture recycled above land are
substantially lower than the mean residence times of total moisture. The
method of age tracers was previously also used by <xref ref-type="bibr" rid="bib1.bibx20" id="text.43"/>, who
found residence times of multiple months. However, <xref ref-type="bibr" rid="bib1.bibx20" id="text.44"/>
started counting from sea evaporation in his experiments and continued the
aging after water precipitated on land, infiltrated into the soil and
re-evaporated. Therefore, his results cannot be interpreted as atmospheric
residence times directly.</p>
      <p>The established knowledge of the residence time of water in the atmosphere
being 8–10 days was recently challenged by <xref ref-type="bibr" rid="bib1.bibx17" id="text.45"/>. They used
backward trajectories computed by  Lagrangian particle tracking
method FLEXPART (forced
with ERA-I) and concluded that the global mean residence time of water in the
atmosphere is 4–5 days, i.e., half of the traditional estimates. More
precisely, they calculated the residence time to be 3.9 <inline-formula><mml:math id="M14" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8 days
(spatial variability indicated by 1 standard deviation) for 15-day backward
trajectories and 4.4 days for 20-day backward trajectories, and showed
spatial figures of the first estimate. An obvious candidate for the
discrepancy with the prevailing knowledge is the length of their
trajectories; however, they stated that almost 100 % of the original
moisture can be attributed to evaporation after 20 days, and that further
backtracking is unphysical and can never come close to the 8–10-day
estimate. Here, we would like to point out another important assumption,
which was not addressed by <xref ref-type="bibr" rid="bib1.bibx17" id="text.46"/>, namely that their
methodology can accurately estimate evaporation. It should be known that
FLEXPART is generally only used to look at specific humidity changes
(evaporation <inline-formula><mml:math id="M15" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula> precipitation, or <inline-formula><mml:math id="M16" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula> <inline-formula><mml:math id="M17" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M18" display="inline"><mml:mi>P</mml:mi></mml:math></inline-formula>). Attribution of
evaporation is difficult as <xref ref-type="bibr" rid="bib1.bibx25" id="text.47"/> note that a number of
moisture transport processes are neglected, which are moisture changes due to
convection, turbulence, numerical diffusion, and rainwater evaporation.
<xref ref-type="bibr" rid="bib1.bibx27" id="text.48"/> even note that specific humidity fluctuations along a
trajectory may be entirely unphysical. <xref ref-type="bibr" rid="bib1.bibx26" id="text.49"/>, who evaluated the
FLEXPART methodology, found that when FLEXPART is used to evaluate <inline-formula><mml:math id="M19" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula>
and <inline-formula><mml:math id="M20" display="inline"><mml:mi>P</mml:mi></mml:math></inline-formula> separately, evaporation is highly overestimated. Specifically, they
obtained a global average evaporation of <inline-formula><mml:math id="M21" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula> <inline-formula><mml:math id="M22" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 1380 mm yr<inline-formula><mml:math id="M23" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, which
corresponds to <inline-formula><mml:math id="M24" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula> <inline-formula><mml:math id="M25" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 704 <inline-formula><mml:math id="M26" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<inline-formula><mml:math id="M27" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> km<inline-formula><mml:math id="M28" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> yr<inline-formula><mml:math id="M29" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. Using
the numbers obtained by Stohl and James (2004) and ERA-Interim atmospheric
storage, a global average residence time of
12.4 <inline-formula><mml:math id="M30" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<inline-formula><mml:math id="M31" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> km<inline-formula><mml:math id="M32" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> / 704 <inline-formula><mml:math id="M33" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<inline-formula><mml:math id="M34" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> km<inline-formula><mml:math id="M35" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> yr<inline-formula><mml:math id="M36" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M37" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 0.017 years <inline-formula><mml:math id="M38" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 6.4 days
is obtained. Overestimation of evaporation will thus bias the estimates of
residence times downward. How this assumption influences the results by LS16
was not evaluated in their paper. Whatever the methodological reason for the
low global mean residence time estimates by <xref ref-type="bibr" rid="bib1.bibx17" id="text.50"/>, we will
argue in this paper that these numbers are physically impossible.</p>
      <p>The objective of this paper is to revisit the current knowledge and provide a
state-of-the-art view in time and space of the residence time of water in the
atmosphere using several different approaches. Table 1 provides a
non-exhaustive overview of the global average residence time of water in the
atmosphere found by the studies mentioned in this introduction. Section 2
explains the methods used in this study. In Sect. 3 we explain why the global
average residence time estimates based on quantifications of the global
hydrological cycle are valid and the counterarguments provided by
<xref ref-type="bibr" rid="bib1.bibx17" id="text.51"/> are not. In Sect. 4 we provide near-global spatial
pictures of atmospheric residence time above land and sea. Section 5 analyzes
the probability density function of the residence time of atmospheric water
particles, and, finally, in Sect. 6 we state the conclusions of this paper.</p>
</sec>
<sec id="Ch1.S2">
  <title>Methods</title>
<sec id="Ch1.S2.SS1">
  <title>Global hydrological data</title>
      <p>In this paper we use flux estimates of the global hydrological cycle as
provided by <xref ref-type="bibr" rid="bib1.bibx21" id="text.52"/>. More specifically, we use the estimates of
<xref ref-type="bibr" rid="bib1.bibx21" id="text.53"/> that were optimized by forcing water and energy budget
closure, taking into account uncertainty in the original estimates. For the
estimation of precipitable water in the atmosphere we use the average of
eight reanalysis datasets provided by <xref ref-type="bibr" rid="bib1.bibx31" id="text.54"/> and we estimate
uncertainty therein by calculating the variance of the eight datasets
assuming equal probability. The data describe the period of 2002–2008
<xref ref-type="bibr" rid="bib1.bibx31" id="paren.55"/> and the period of approximately the first decade of the
21st century <xref ref-type="bibr" rid="bib1.bibx21" id="paren.56"/>, respectively, but in the latter case it
depends on the underlying input data. Moreover, we use global ERA-I
precipitation and evaporation for the period 2002–2008 to compute the
results based on ERA-I only.</p><?xmltex \hack{\newpage}?>
</sec>
<sec id="Ch1.S2.SS2">
  <title>Moisture tracking models</title>
      <p>We use two different moisture tracking models, namely WAM-2layers (Water
Accounting Model – 2 layers) <xref ref-type="bibr" rid="bib1.bibx35 bib1.bibx36" id="paren.57"/> and 3D-T
(3-Dimensional – Trajectories) <xref ref-type="bibr" rid="bib1.bibx32" id="paren.58"/> based on
<xref ref-type="bibr" rid="bib1.bibx6" id="text.59"/>. These models are Eulerian and Lagrangian offline
moisture tracking models, respectively, and we refer to their respective
references for a detailed description. Both models track tagged water
through the atmosphere from its source
(evaporation) to its sink (precipitation), or reverse when tracking
precipitation back in time to the place where it evaporated. The most
important assumption in both models is that precipitation stems from the
entire atmospheric column (humidity-weighted). Both models are improved from
earlier versions and were validated against a detailed online moisture
tracking method within a regional climate model <xref ref-type="bibr" rid="bib1.bibx15 bib1.bibx40" id="paren.60"/>. We force the models with global ERA-I data from which we use
2-D fields of 3-hourly precipitation and evaporation, 6-hourly surface
pressure, specific humidity and zonal and meridional wind speed on model
levels covering the entire atmosphere from zero to surface pressure.
Additionally, for 3D-T, we use 6-hourly vertical wind speeds on model levels.
We use and present the data for the period 2002–2008, exactly corresponding
to the period studied by <xref ref-type="bibr" rid="bib1.bibx31" id="text.61"/> and approximately the period
studied by <xref ref-type="bibr" rid="bib1.bibx21" id="text.62"/>. For both models we use computational time
steps of 0.25 h. For WAM-2layers we use 1 additional year at the beginning
or end of this period for spin-up and a grid size of
1.5<inline-formula><mml:math id="M39" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> latitude <inline-formula><mml:math id="M40" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 1.5<inline-formula><mml:math id="M41" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> longitude. Vertical exchange
between the two layers is parametrized and tagged water is not allowed to
exceed the total water in the column. In the Lagrangian moisture tracking
model we use a finer resolution, 0.25<inline-formula><mml:math id="M42" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M43" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 0.25<inline-formula><mml:math id="M44" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, and
we release one parcel every hour for each grid cell at a random horizontal
location. The initial vertical location of a released parcel is 50 hPa above
the land surface in the forward tracking scheme and humidity-weighted random
in the backward tracking scheme. Some sensitivity tests on the number of
parcels released showed that the release of one parcel per hour yielded
stable results in terms of determining the residence time. Note that the
validity of spatial and temporal variability in the results (Sects. 4 and 5)
depends strongly on how well ERA-I is able to describe the hydrological
cycle.</p>
<sec id="Ch1.S2.SS2.SSS1">
  <title>Experiments with WAM-2layers</title>
      <p>The model calculates the age <inline-formula><mml:math id="M45" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi>g</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of the tagged moisture present in a
grid cell layer according to the following formula:

                  <disp-formula id="Ch1.E1" content-type="numbered"><mml:math id="M46" display="block"><mml:mstyle class="stylechange" displaystyle="true"/><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><?xmltex \hack{\hbox\bgroup\fontsize{7}{7}\selectfont$\displaystyle}?><mml:msubsup><mml:mi>N</mml:mi><mml:mi>g</mml:mi><mml:mi>t</mml:mi></mml:msubsup><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mfenced close=")" open="("><mml:mtable class="array" columnalign="left"><mml:mtr><mml:mtd><mml:mrow><mml:msubsup><mml:mi>W</mml:mi><mml:mi>g</mml:mi><mml:mrow><mml:mi>t</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msubsup><mml:mfenced close=")" open="("><mml:msubsup><mml:mi>N</mml:mi><mml:mi>g</mml:mi><mml:mrow><mml:mi>t</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msubsup><mml:mo>+</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi></mml:mfenced><mml:mo>+</mml:mo><mml:mo>∑</mml:mo><mml:msub><mml:mi>F</mml:mi><mml:mrow><mml:mi>g</mml:mi><mml:mo>,</mml:mo><mml:mtext>in</mml:mtext></mml:mrow></mml:msub><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:mfenced close=")" open="("><mml:msubsup><mml:mi>N</mml:mi><mml:mrow><mml:mi>g</mml:mi><mml:mo>,</mml:mo><mml:mtext>in</mml:mtext></mml:mrow><mml:mrow><mml:mi>t</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msubsup><mml:mo>+</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi></mml:mfenced></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mrow><mml:mo>-</mml:mo><mml:mo>∑</mml:mo><mml:msub><mml:mi>F</mml:mi><mml:mrow><mml:mi>g</mml:mi><mml:mo>,</mml:mo><mml:mtext>out</mml:mtext></mml:mrow></mml:msub><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:mfenced open="(" close=")"><mml:msubsup><mml:mi>N</mml:mi><mml:mi>g</mml:mi><mml:mrow><mml:mi>t</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msubsup><mml:mo>+</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi></mml:mfenced><mml:mo>-</mml:mo><mml:msub><mml:mi>P</mml:mi><mml:mi>g</mml:mi></mml:msub><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:mfenced close=")" open="("><mml:msubsup><mml:mi>N</mml:mi><mml:mi>g</mml:mi><mml:mrow><mml:mi>t</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msubsup><mml:mo>+</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi></mml:mfenced><mml:mo>+</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi>g</mml:mi></mml:msub><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:mfrac></mml:mstyle></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mfenced></mml:mrow><mml:mrow><mml:msubsup><mml:mi>W</mml:mi><mml:mi>g</mml:mi><mml:mi>t</mml:mi></mml:msubsup></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo><?xmltex \hack{$\egroup}?></mml:mrow></mml:math></disp-formula>

            <?xmltex \hack{\newpage}?><?xmltex \hack{\noindent}?>where the subscript “<inline-formula><mml:math id="M47" display="inline"><mml:mi>g</mml:mi></mml:math></inline-formula>” stands for tagged water. The superscripts “<inline-formula><mml:math id="M48" display="inline"><mml:mi>t</mml:mi></mml:math></inline-formula>”
and “<inline-formula><mml:math id="M49" display="inline"><mml:mi>t</mml:mi></mml:math></inline-formula> <inline-formula><mml:math id="M50" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula> 1” are the current and previous time steps, respectively.
<inline-formula><mml:math id="M51" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi></mml:mrow></mml:math></inline-formula> is the length of the time step. <inline-formula><mml:math id="M52" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mrow><mml:mi>g</mml:mi><mml:mo>,</mml:mo><mml:mtext>in</mml:mtext></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> stands for the
age of the tagged water coming into the grid cell layer.
<inline-formula><mml:math id="M53" display="inline"><mml:mrow><mml:msub><mml:mi>F</mml:mi><mml:mrow><mml:mi>g</mml:mi><mml:mo>,</mml:mo><mml:mtext>in</mml:mtext></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M54" display="inline"><mml:mrow><mml:msub><mml:mi>F</mml:mi><mml:mrow><mml:mi>g</mml:mi><mml:mo>,</mml:mo><mml:mtext>out</mml:mtext></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> are the incoming and outgoing fluxes
over the (vertical and horizontal) boundaries of a grid cell layer.</p>
      <p>With WAM-2layers we perform four experiments. In the first experiment we
track continentally evaporated water over the globe until it precipitates and
explicitly calculate the average age in each model layer of each grid cell at
every time step. In the second experiment we do exactly the same, but now we
backtrack continental precipitation to its origin. The third and fourth
experiments are equal to the first and second, but now for tracking of
oceanic evaporation and precipitation, respectively.</p>
      <p>The combined continental and oceanic tracking results are used to obtain
global estimates (see Fig. 1) as well as spatial pictures of residence time
and age of water in the atmosphere (see Figs. 2, 3, and S1 in the
Supplement). WAM-2layers does not work well with very small grid cells near
the poles (time steps need to be very small to ensure stability, due to the
explicit scheme used); thus, we use data only between 80<inline-formula><mml:math id="M55" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S and
80<inline-formula><mml:math id="M56" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N (missing about 1 % of the Earth's surface), and present our
results between 75<inline-formula><mml:math id="M57" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S and 75<inline-formula><mml:math id="M58" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N (missing less than 3 % of
the Earth's surface). Tagged water crossing these boundaries is considered
lost. For the global water balance calculations we do include data from the
entire Earth, but evaporation and precipitation are very low at these high
latitudes (about 0.2 % of the global hydrological cycle) and, thus, do not
affect the results very much.</p>
</sec>
<sec id="Ch1.S2.SS2.SSS2">
  <title>Experiments with 3D-T</title>
      <p>With the Lagrangian moisture-tracking model, we perform a forward experiment
and a backward experiment. In the forward experiment, evaporation parcels
from the Earth's surface are tracked through the atmosphere forward in time
to their next precipitation location. In the backward experiment,
precipitation parcels are tracked backward in time to their previous
evaporation location.</p>
      <p>Every time a moisture parcel (either evaporation or precipitation) is tracked
forward or backward, its moisture balance is made during every time step. As
a result of this moisture balance, we allocate a fraction of the original
moisture to leave the atmospheric water cycle at that location. For example,
in the forward experiment, we allocate a part of the evaporated water to each
precipitation event located along the moisture trajectory. This procedure
provides a probability density of the atmospheric residence time of the
evaporation that is tracked forward or the precipitation that is tracked
backward. The moisture is followed through the atmosphere during a period of
30 days, and, the residence time is accounted for the volume of
moisture that leaves the atmosphere. After 30 days of tracking, if
there is moisture that is unaccounted for, it is assumed to have a residence
time of 30 days.</p>
      <p>For each 0.25<inline-formula><mml:math id="M59" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> grid cell (see Figs. 2, 3, and S1), these probability
densities (see Fig. 4) are summed for all time steps during 2002–2008,
weighted by the amount of evaporation or precipitation during the time of
release. To acquire a global mean residence time, the global means of local
mean residence times are determined by weighting by total evaporation or
precipitation volume (see Fig. 1).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F1" specific-use="star"><caption><p>Earth's hydrological cycle with residence times (2002–2008). All
residence times shown are weighted averages. The uncertainty ranges indicated
for the residence times from the moisture tracking methods refer to the
uncertainty associated with model choice (WAM-2layers or 3D-T). Tre11 stands
for <xref ref-type="bibr" rid="bib1.bibx31" id="text.63"/> and Rod15 stands for <xref ref-type="bibr" rid="bib1.bibx21" id="text.64"/>. The land
area is 147 <inline-formula><mml:math id="M60" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<inline-formula><mml:math id="M61" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">6</mml:mn></mml:msup></mml:math></inline-formula> km<inline-formula><mml:math id="M62" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula> and the ocean area is
363 <inline-formula><mml:math id="M63" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<inline-formula><mml:math id="M64" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">6</mml:mn></mml:msup></mml:math></inline-formula> km<inline-formula><mml:math id="M65" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>.</p></caption>
            <?xmltex \igopts{width=412.564961pt}?><graphic xlink:href="https://hess.copernicus.org/articles/21/779/2017/hess-21-779-2017-f01.pdf"/>

          </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F2" specific-use="star"><caption><p>Annual average hydrological cycle, atmospheric residence times and
age for 2002–2008, based on ERA-Interim data. <bold>(a)</bold> Precipitation,
<bold>(b)</bold> evaporation, <bold>(c)</bold> weighted average atmospheric residence
time of precipitation (average of WAM-2layers and 3D-T),
<bold>(d)</bold> weighted average atmospheric residence time of precipitation
(average of WAM-2layers and 3D-T), and <bold>(e)</bold> time-averaged age of
atmospheric water as it is the atmospheric column (WAM-2layers). The arrows
indicate the vertically integrated moisture fluxes. <bold>(f)</bold> Latitudinal
averages. The individual estimates from WAM-2layers and 3D-T for <bold>(c)</bold>
and <bold>(d)</bold> can be found in the Supplement (Fig. S1). The age of
atmospheric water <bold>(e)</bold> for all days individually can also be found in
the Supplement (Animation 1).</p></caption>
            <?xmltex \igopts{width=483.69685pt}?><graphic xlink:href="https://hess.copernicus.org/articles/21/779/2017/hess-21-779-2017-f02.png"/>

          </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F3" specific-use="star"><caption><p>Time metrics in January and July. <bold>(a)</bold> Time-averaged age of
atmospheric water in January (2002–2008) as computed by WAM-2layers based on
ERA-Interim data. The arrows indicate the vertically integrated moisture fluxes.
<bold>(b)</bold> Latitudinal averages of residence times and water age in January.
<bold>(c)</bold> As <bold>(a)</bold> for July. <bold>(d)</bold> As <bold>(b)</bold> for July.
The spatial residence time figures for January and July can be found in the
Supplement (Fig. S2).</p></caption>
            <?xmltex \igopts{width=483.69685pt}?><graphic xlink:href="https://hess.copernicus.org/articles/21/779/2017/hess-21-779-2017-f03.png"/>

          </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F4" specific-use="star"><caption><p>Probability density functions (PDFs) of atmospheric residence time
as computed by 3D-T based on ERA-Interim data (2002–2008). <bold>(a)</bold> PDFs
of precipitation residence time, and <bold>(b)</bold> PDFs of evaporation
residence time. About 5 % of the moisture has residence times of more than
30 days.</p></caption>
            <?xmltex \igopts{width=398.338583pt}?><graphic xlink:href="https://hess.copernicus.org/articles/21/779/2017/hess-21-779-2017-f04.png"/>

          </fig>

</sec>
</sec>
</sec>
<sec id="Ch1.S3">
  <title>Why the global average residence time of water in the atmosphere is 8–10 days</title>
      <p>If one would like to know the average residence time <inline-formula><mml:math id="M66" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula> in any reservoir,
one simply divides its average mass <inline-formula><mml:math id="M67" display="inline"><mml:mover accent="true"><mml:mi>M</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> (or volume when assuming
constant density) by its average outgoing mass flux <inline-formula><mml:math id="M68" display="inline"><mml:mover accent="true"><mml:mi>F</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> (which
equals the ingoing flux when there is no change in mass):

              <disp-formula id="Ch1.E2" content-type="numbered"><mml:math id="M69" display="block"><mml:mstyle displaystyle="true" class="stylechange"/><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mover accent="true"><mml:mi>M</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mover accent="true"><mml:mi>F</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:mfrac></mml:mstyle><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>

        While this is a simple formula, computation of reliable residence times in,
for example, a surface water lake may be difficult due to many uncertainties
in a lake's volume, hydraulic flow, precipitation, evaporation and seepage
<xref ref-type="bibr" rid="bib1.bibx18" id="paren.65"><named-content content-type="pre">e.g.,</named-content></xref>. Moreover, a lake may be permanently stratified
(i.e., there is permanent dead storage), and one could argue that the actual
volume participating in the water cycle of the lake does not equal the lake's
total volume, meaning that the actual average residence time becomes lower.
If one can, however, reliably estimate a lake's volume and inflow or outflow,
it is not necessary for a lake to be well mixed for Eq. (2) to hold, nor is
it necessary for <inline-formula><mml:math id="M70" display="inline"><mml:mi>F</mml:mi></mml:math></inline-formula> to be constant. The mere necessity is that the entire
volume participates in the water cycle. Of course, one could still have
significant local differences, but the average can reliably be calculated by
Eq. (2).</p>
      <p>When the Earth's entire atmosphere is considered to be the reservoir of
study, its residence time can actually be calculated much more easily than
that of a lake. In the global case the only inflow is evaporation and the
only outflow is precipitation. Moreover, due to the turbulent nature of the
atmosphere all water that resides in the atmosphere also participates in the
atmospheric water cycle; i.e., there is no such thing as permanent dead water
storage <xref ref-type="bibr" rid="bib1.bibx13" id="paren.66"><named-content content-type="pre">e.g.,</named-content></xref>. This is furthermore supported by the
online passive moisture tracking experiments of <xref ref-type="bibr" rid="bib1.bibx2" id="text.67"/>. Note
that this online tracking method does not suffer from the well-mixed
assumption for precipitation. Even so, they found that by tagging all
moisture in the atmosphere, after 30 days, there was only 3 % of the tagged
passive moisture left; thus, at least 97 % of the total moisture in the
atmosphere must have been participating in the hydrological cycle within
30 days.</p>
      <p><?xmltex \hack{\newpage}?>The use of Eq. (2) to calculate the global mean residence time of atmospheric
water has recently been criticized by <xref ref-type="bibr" rid="bib1.bibx17" id="text.68"/>. They argued that
Eq. (2) is (a) not a reliable estimator for local residence times as it does
not involve horizontal moisture transport, (b) should be corrected for the
surface area of the Earth where most
precipitation is observed, and (c) that the temporal characteristics of
global precipitation cannot be measured by depletion time constants. However,
we disagree with these arguments as (a<inline-formula><mml:math id="M71" display="inline"><mml:msup><mml:mi/><mml:mo>*</mml:mo></mml:msup></mml:math></inline-formula>) horizontal moisture transport
is irrelevant for the global average value, (b<inline-formula><mml:math id="M72" display="inline"><mml:msup><mml:mi/><mml:mo>*</mml:mo></mml:msup></mml:math></inline-formula>) the surface area of the
Earth is irrelevant as it is not in Eq. (2), but nonetheless all areas
participate in the hydrological cycle as there is also transport even over
the Sahara <xref ref-type="bibr" rid="bib1.bibx11 bib1.bibx23" id="paren.69"><named-content content-type="pre">e.g.,</named-content></xref>, and (c<inline-formula><mml:math id="M73" display="inline"><mml:msup><mml:mi/><mml:mo>*</mml:mo></mml:msup></mml:math></inline-formula>) the
values in Eq. (2) correspond to the elemental physical concept that an
average residence time can be calculated from dividing a stock by its average
influx or outflux under the assumption that there is negligible net stock
change over a longer period; whether these average fluxes are constant or not
is irrelevant, and the temporal characteristics of precipitation and
evaporation can only affect the probability density functions of the
residence time (Sect. 5), but not the average. In the Supplement we dispute
the counterexamples, objecting to Eq. (2) by <xref ref-type="bibr" rid="bib1.bibx17" id="text.70"><named-content content-type="post">Supplement
Sect. 4</named-content></xref>, in more detail. Moreover, we argued above that the
entire atmospheric volume participates in the hydrological cycle. Thus,
Eq. (2) can, in our opinion, safely be used to calculate the global average
residence time of atmospheric water.</p>
      <p>Applying Eq. (2) to estimates of the global hydrological cycle (Fig. 1)
yields a global mean residence time of atmospheric water of
8.9 <inline-formula><mml:math id="M74" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4 days (uncertainty indicated by 1 standard deviation). The
calculation of the mean is as follows:

              <disp-formula id="Ch1.E3" content-type="numbered"><mml:math id="M75" display="block"><mml:mstyle class="stylechange" displaystyle="true"/><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mn>12.6</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow><mml:mrow><mml:mo>(</mml:mo><mml:mn>403.5</mml:mn><mml:mo>+</mml:mo><mml:mn>116.5</mml:mn><mml:mo>)</mml:mo><mml:mo>×</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>=</mml:mo><mml:mn>0.024</mml:mn><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mtext>years</mml:mtext><mml:mo>=</mml:mo><mml:mn>8.9</mml:mn><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mtext>days</mml:mtext><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>

        and the standard deviation was calculated by general uncertainty propagation
theory. The 1st and 99th percentiles of this estimate are 7.9 and 9.8 days,
respectively. All previous global average estimates referred to in this paper
roughly fall within this uncertainty range (Table 1), except for the estimate
provided by <xref ref-type="bibr" rid="bib1.bibx17" id="text.71"/>, which is less than half. Based on the
arguments provided in this section we believe that the latter estimate is
incorrect (the probability of an atmospheric residence time lower than
3.9 days equals 1 <inline-formula><mml:math id="M76" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<inline-formula><mml:math id="M77" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn>30</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). Even if we make the assumption that
water outside the troposphere, and thus in the stratosphere or mesosphere
(where aerosol lifetimes on the order of 1 year have been found;
<xref ref-type="bibr" rid="bib1.bibx16" id="altparen.72"/>), does not participate in the hydrological cycle,
the atmospheric storage is reduced by <inline-formula><mml:math id="M78" display="inline"><mml:mo>∼</mml:mo></mml:math></inline-formula> 1 % only. The corresponding
global average residence time of water in the troposphere then is
8.8 <inline-formula><mml:math id="M79" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4 days, and thus nowhere near the estimates by
<xref ref-type="bibr" rid="bib1.bibx17" id="text.73"/>. In the following example we show that their findings
violate global mass balance: let us start from the fact that the average
atmospheric water storage in ERA-I is 12.4 <inline-formula><mml:math id="M80" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<inline-formula><mml:math id="M81" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> km<inline-formula><mml:math id="M82" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> and
the average precipitation rate in ERA-I is
531 <inline-formula><mml:math id="M83" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<inline-formula><mml:math id="M84" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> km<inline-formula><mml:math id="M85" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> yr<inline-formula><mml:math id="M86" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M87" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 1.45 <inline-formula><mml:math id="M88" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<inline-formula><mml:math id="M89" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> km<inline-formula><mml:math id="M90" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> day<inline-formula><mml:math id="M91" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M92" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 2.85 mm day<inline-formula><mml:math id="M93" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (Fig. 1). For the sake of the example, let us neglect the 1 %
moisture outside the troposphere. Then, the resulting active atmospheric
storage is 12.3 <inline-formula><mml:math id="M94" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<inline-formula><mml:math id="M95" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> km<inline-formula><mml:math id="M96" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula>. For that atmospheric water to
have a residence time of 3.9 days, there must have been an evaporation rate
of
12.3 <inline-formula><mml:math id="M97" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<inline-formula><mml:math id="M98" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula>/3.9 <inline-formula><mml:math id="M99" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 3.15 <inline-formula><mml:math id="M100" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<inline-formula><mml:math id="M101" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> km<inline-formula><mml:math id="M102" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> day<inline-formula><mml:math id="M103" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M104" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 6.03 mm day<inline-formula><mml:math id="M105" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>,
which is physically impossible as that means an enormous imbalance in <inline-formula><mml:math id="M106" display="inline"><mml:mi>P</mml:mi></mml:math></inline-formula>
and <inline-formula><mml:math id="M107" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula>. Alternatively, it would require an enormous part of the atmospheric
water to be dead storage (i.e., never participate in the hydrological cycle),
namely
12.4 <inline-formula><mml:math id="M108" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<inline-formula><mml:math id="M109" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M110" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula> 1.45 <inline-formula><mml:math id="M111" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<inline-formula><mml:math id="M112" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M113" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 3.9 <inline-formula><mml:math id="M114" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 6.7 <inline-formula><mml:math id="M115" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 10<inline-formula><mml:math id="M116" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> km<inline-formula><mml:math id="M117" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula>
or 54 % of all water in the atmosphere.</p>
      <p>Figure 1 shows several estimates of global residence times. ERA-I fluxes fall
well within the uncertainty ranges provided by <xref ref-type="bibr" rid="bib1.bibx21" id="text.74"/>, but they
are generally on the high side. Thus, the global mean residence time estimate
of 8.4–8.6 days, based on global ERA-I data, is slightly on the low
side of the uncertainty spectrum. The estimates from our moisture tracking
methods (WAM-2layers and 3D-T), which use ERA-I, match quite well for global
mean atmospheric residence time. The moisture tracking estimates split out
for land and ocean are, therefore, slightly lower than the most likely value
of 8.9 days. However, it is clear that the turnover of water in the
atmosphere is faster over the ocean than over land, having a difference of
about 2 days. The logical explanation here is that the hydrological
cycle over the ocean is not limited by dry conditions on land, and, as a
consequence, is more intense.</p>
</sec>
<sec id="Ch1.S4">
  <title>A spatial view of the residence time of atmospheric moisture</title>
      <p>Figure 2 provides a near-global spatial view of the annual average
hydrological cycle, atmospheric residence times and age. Globally averaged,
precipitation residence time, evaporation residence time and age of
atmospheric water should be the same, but may differ due to imbalances in the
data of the atmospheric hydrological cycle (see Fig. 1). More importantly,
these three metrics have a different physical meaning, and thus, a different
spatial pattern (Fig. 2c–e). Let us consider a particular location in the
world, in this case Portugal, as an example. As can be seen from Fig. 2d,
moisture which evaporates from Portugal stays in the atmosphere on average
about 14–15 days before it rains out again. In other words: the atmospheric
residence time of evaporation is 14–15 days. The local recycling of
atmospheric water is only a few percent <xref ref-type="bibr" rid="bib1.bibx7 bib1.bibx37" id="paren.75"><named-content content-type="pre">e.g.,</named-content></xref>, and much of the evaporated atmospheric moisture is, in fact,
transported towards relatively dry regions in the Mediterranean and Africa
<xref ref-type="bibr" rid="bib1.bibx23 bib1.bibx39" id="paren.76"><named-content content-type="pre">e.g.,</named-content></xref>, hence the relatively long
atmospheric residence time of evaporation. On the other hand, the
precipitation in Portugal comes for a large part from oceanic sources
relatively nearby <xref ref-type="bibr" rid="bib1.bibx7 bib1.bibx9 bib1.bibx38" id="paren.77"><named-content content-type="pre">e.g.,</named-content></xref>, and we estimate that is has resided in the atmosphere for
about 7–8 days (Fig. 2c) before it fell as precipitation in Portugal. In
other words: the atmospheric residence time of precipitation is 7–8 days.
The spatial image of the age of atmospheric water (Fig. 2e) is very similar
to the precipitation residence time (Fig. 2c). For our Portugal example, the
average age of atmospheric water is about about 8–10 days. Precipitation
draws its water from the atmospheric reservoir with a certain age, but
apparently, the atmospheric moisture in the drier months has a higher age.
Hence, for Portugal, the time-averaged age of atmospheric moisture can be
somewhat higher than the precipitation-weighted atmospheric residence time of precipitation.</p>
      <p>With Fig. 2 we would like to stress that there are multiple ways of looking
at the residence of atmospheric moisture. Whether you look at residence time
from a precipitation perspective (Fig. 2c) or an evaporation perspective
(Fig. 2d) gives an entirely different picture. In the precipitation
perspective, the time from the previous evaporation is stressed, while in the
evaporation perspective, the time to the next precipitation event is
stressed. The definition of an atmospheric residence time – for both
precipitation and evaporation – is analogous to the definition of other
metrics for the atmospheric branch of the hydrological cycle, which are also
defined for both the precipitation and evaporation perspectives <xref ref-type="bibr" rid="bib1.bibx28 bib1.bibx29 bib1.bibx39 bib1.bibx37" id="paren.78"><named-content content-type="pre">e.g.,</named-content></xref>. Moreover,
you can also look at the actual age of atmospheric water as it resides in the
atmosphere (Fig. 2e). Figure 2f provides the latitudinal averages of
Fig. 2c–e, as well as of the estimates from WAM-2layers and 3D-T separately
(Fig. S1), for which a discussion is attached in the Supplement.</p>
      <p>Figure 2c is directly comparable to a recent estimate
<xref ref-type="bibr" rid="bib1.bibx17" id="paren.79"><named-content content-type="post">Fig. 2a</named-content></xref>. Their spatial patterns are very similar,
however, we observe that they underestimate the residence time everywhere
with a factor 2–3 compared to our results. As pointed out in the
introduction, the method of <xref ref-type="bibr" rid="bib1.bibx17" id="text.80"/> relies on the unevaluated
assumption that they can accurately attribute evaporation, and on a rather
short length of their trajectories (15 or 20 days). In contrast, our
methods use longer trajectories (WAM-2layers: continuous; 3D-T:
30 days), and use the fields of ERA-I evaporation directly. Moreover,
our global average values fit with the atmospheric water balance (Eq. 2 and
Fig. 1). For an extensive discussion of the counterarguments of
<xref ref-type="bibr" rid="bib1.bibx17" id="text.81"/> against the use of Eq. (2), and our rebuttal, we would
like to refer the reader to the Supplement attached to this paper.</p>
      <p>We make the following observations based on Fig. 2.
<list list-type="bullet"><list-item>
      <p>The places of low precipitation residence times (Fig. 2c) coincide mostly
with areas of low precipitation (Fig. 2a). This indicates that if there is
precipitation, its water content has recently evaporated and is most likely
of local origin. Note that the reverse statement, low precipitation (Fig. 2a)
coinciding with low precipitation residence times (Fig. 2c), is not
necessarily true.</p></list-item><list-item>
      <p>The intertropical convergence zone (ITCZ) has increasing precipitation
residence times (Fig. 2c) and decreasing evaporation residence times
(Fig. 2d) towards its center. This holds over the ocean as well as over the
northern Amazon and Indonesia. The atmospheric residence time of evaporation
(Fig. 2d) can often be seen as an indication of the moisture travel distance
towards an area of high precipitation such as the ITCZ.</p></list-item><list-item>
      <p>The Southern Hemisphere ocean (roughly between 45 and 75<inline-formula><mml:math id="M118" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S) has
evaporation residence times (Fig. 2d) of less than 5 days, while absolute
evaporation is low (Fig. 2b). This can be explained by relatively high precipitation
rates (Fig. 2a) compared to the amount of atmospheric water vapor that is in the air
<xref ref-type="bibr" rid="bib1.bibx19" id="paren.82"><named-content content-type="pre">e.g.,</named-content></xref>, so evaporation has a quick turnover.</p></list-item><list-item>
      <p>Over the Sahara, the age of atmospheric water (Fig. 2e) as well as residence
times (Fig. 2c and d) are more than 15 days, indicating that moisture comes from
remote sources. Over the Tibetan Plateau there is a reversed situation where
the age of atmospheric water and residence times are low relative to surrounding values.
<?xmltex \hack{\newpage}?></p></list-item><list-item>
      <p>When following the atmospheric moisture flow inland from the coast, the age
of atmospheric water increases (Fig. 2e), as does the residence time of
precipitation. This feature is very clear over Eurasia, but can be observed on
other continents as well.</p></list-item><list-item>
      <p>Latitudinally averaged (Fig. 2f), the precipitation residence time peaks
towards the poles and the Equator. This is in anticorrelation with the
residence time of evaporation. This corresponds to the Hadley and Ferrel
cells, transporting evaporated atmospheric moisture from the high-pressure
zones with the prevailing trade winds and westerlies towards areas of high
precipitation.</p></list-item></list></p>
      <p>Figure 3 shows the age and residence times of atmospheric water in January
and July. In January (Fig. 3a) the age of atmospheric water is relatively low
in the Northern Hemisphere, and relatively high in the Southern Hemisphere.
In July (Fig. 3c) the pattern is reversed. In much of the Southern Hemisphere
the atmospheric moisture storage (see Fig. S3) is lower in July (Fig. S3b)
compared to January (Fig. S3a), precipitates rates are higher in July
(Fig. S3d) compared to January (Fig. S3c), and evaporation rates are also
higher in July (Fig. S3f) compared to January (Fig. S3e). The higher
evaporation rates in July in the ERA-I data may seem counterintuitive, but
correspond to previous studies <xref ref-type="bibr" rid="bib1.bibx46" id="paren.83"><named-content content-type="pre">e.g.,</named-content></xref>. It is, therefore,
quite logical that lower storage and higher fluxes lead to lower moisture
ages in the Southern Hemisphere in July (Fig. 3c) compared to January
(Fig. 3a). Note that Animation 1 in the Supplement provides a view of
moisture age throughout the year. The seasonal patterns we observe for
precipitation residence times (Fig. S2a and c) are quite similar to
<xref ref-type="bibr" rid="bib1.bibx17" id="text.84"><named-content content-type="post">Fig. S3</named-content></xref>, albeit that their figures are for DJF and
JJA, while ours are for January and July, and, as for the yearly average
figures, their absolute values are much lower.</p>
      <p>Over the continents, especially Eurasia, the pattern of atmospheric water age
is complex, and we observe an interesting ocean-to-land contrast (Fig. 3). In
January, looking at the Northern Hemisphere, the ocean is relatively warm
compared to the land, and the age of atmospheric water increases going
inland, as there is little replenishment from land evaporation. In July the
opposite situation occurs: the ocean is relatively cool compared to the land
and the age of atmospheric water decreases going inland. This corresponds to
high evaporation rates and corresponding high continental moisture recycling
ratios <xref ref-type="bibr" rid="bib1.bibx8 bib1.bibx35" id="paren.85"><named-content content-type="pre">e.g.,</named-content></xref>. As a result, the
atmospheric water age over a large part of Asia is actually lower in July
compared to January. Over the Southern Hemisphere we see the same
ocean-to-land contrast, but it is less pronounced as there is relatively
little land present. The latitudinally averaged residence times of
precipitation and evaporation (Fig. 3b and d) also show the summer vs. winter
reversal.</p><?xmltex \hack{\newpage}?>
</sec>
<sec id="Ch1.S5">
  <title>The probability density function of the residence time of atmospheric moisture</title>
      <p>Figure 4 shows probability density functions (PDFs) for residence times.
Theoretically, the global PDFs of evaporation and precipitation residence
time should be identical. However, they slightly differ, which can be
attributed to inconsistencies in the ERA-I forcing data as well as the
assumptions made in the tracking model. Regarding the forcing data, it seems
from Fig. 1 that the lifetime of atmospheric moisture is slightly too short,
a common issue in all models <xref ref-type="bibr" rid="bib1.bibx30" id="paren.86"/>, indicating that our
results may be slightly skewed towards lower residence times. According to
<xref ref-type="bibr" rid="bib1.bibx30" id="text.87"/>, precipitation also falls too early in the day in all
models, thus the amplitude of residence times over land could also be
affected, but it is unclear to what extent. Regarding the modeling
assumptions, in 3D-T we assume a humidity-weighted well-mixed atmosphere
during precipitation and the starting location of the trajectories is
randomized over the grid cell. These assumption may lead to an
underestimation of the number of water particles that undergo a very fast
cycle, and may, thus, slightly skew our results towards higher residence
times. By definition of mass balance, however, the actual mean of the
distribution should not change. When more water particles undergo a
faster(slower) cycle, as a logical consequence, also more water particles
undergo a slower(faster) cycle. Adding age tracers to online tracking methods
<xref ref-type="bibr" rid="bib1.bibx44" id="paren.88"/>, but then applied to new global methods <xref ref-type="bibr" rid="bib1.bibx24" id="paren.89"><named-content content-type="pre">e.g.,</named-content></xref>,
would allow to check the validity and consequences of these assumptions in more
detail, however, would still depend on the model world.</p>
      <p>Looking at Fig. 4 we see that short residence times have the highest
probability, but there is a long tail with low probabilities and high
residence times. We find the median residence time of precipitation and
evaporation to be 5.7 and 4.6 days, respectively. Thus, the median is about
3 to 4 days less than the mean (see Fig. 1), indicating that the long tails
skew the mean significantly. About 5 % of the moisture has residence times
of more than 30 days, which we assumed to have a residence time of 30 days
when we calculated the mean (Fig. 1). As a consequence, the estimates for the
mean from 3D-T may be slightly lower than the “true” values. It is unclear
how <xref ref-type="bibr" rid="bib1.bibx17" id="text.90"/> have dealt with the unattributed moisture after the
end of their trajectories, but they already attributed 97 % of the initial
precipitation to evaporation after just 15 days in their Lagrangian model. In
Sect. 3, however, we argued that this is physically impossible from a global
mass balance perspective.</p>
      <p>We furthermore observe an interesting daily cycle in the residence time PDFs
over land (Fig. 4), while the general shape of ocean and land PDFs is not
very different when looking at timescales of multiple days. We suggest that
the daily cooling and warming, resulting in a daily cycle of land
evaporation, and a higher likelihood of precipitation occurring towards the
end of the day, cause the daily cycle in the residence time PDFs. This
phenomenon is only visible over land, as here surface cooling and warming
occur with much greater amplitude than over the ocean. These cycles are
still visible after multiple days (Fig. 4).</p>
</sec>
<sec id="Ch1.S6" sec-type="conclusions">
  <title>Conclusions</title>
      <p>In this paper we studied the residence time of water in the atmosphere. We
revisited the state-of-the-art knowledge and studied its properties in time
and space on a global scale. As discussed in previous sections, our results
are naturally limited by the validity of the input data and the assumptions
in our tracking models. However, we trust our results enough to draw the
following main conclusions.
<list list-type="bullet"><list-item>
      <p>Given the state-of-the-art estimates of the hydrological cycle, the global
mean residence time of atmospheric water is 8.9 <inline-formula><mml:math id="M119" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4 days (uncertainty
indicated by 1 standard deviation). The 1st and 99th percentiles of this
estimate are 7.9 and 9.8 days, respectively.</p></list-item><list-item>
      <p>The average atmospheric residence time over the ocean is about 2 days
less than over land.</p></list-item><list-item>
      <p>Locally, there are different perspectives of looking at residence time.
Atmospheric residence time of evaporation can often be seen as an indication
of the moisture travel distance towards an area of high precipitation such as
the ITCZ, while atmospheric residence time of precipitation is often more complex.</p></list-item><list-item>
      <p>Latitudinally averaged, the residence time of precipitation peaks towards the
poles and the Equator, which is in anticorrelation with the residence time of
evaporation.</p></list-item><list-item>
      <p>In winter, the age of atmospheric water is generally several days less
than in summer.</p></list-item><list-item>
      <p>In the Northern Hemisphere, following atmospheric moisture inland, the age of
atmospheric water increases when the sea is relatively warm compared to the
land and decreases when the sea is relatively cold. This cannot clearly be
observed in the Southern Hemisphere, where less continental mass is present.</p></list-item><list-item>
      <p>Probability density functions of atmospheric residence time have long tails,
with a global median of around 5 days.</p></list-item></list></p>
</sec>
<sec id="Ch1.S7">
  <title>Data availability</title>
      <p>The underlying ERA-Interim data are supplied by ECMWF and can be accessed at
<uri>http://apps.ecmwf.int/datasets/data/interim-full-daily/</uri>. The model code
to reproduce the results is accessible in the following way: the basic code for
WAM-2layers is available for download from Github (van der Ent, 2016), and the
code for 3D-T is available upon request from Obbe Tuinenburg (o.a.tuinenburg@uu.nl).</p>
</sec>

      
      </body>
    <back><app-group>
        <supplementary-material position="anchor"><p><bold>The Supplement related to this article is available online at <inline-supplementary-material xlink:href="http://dx.doi.org/10.5194/hess-21-779-2017-supplement" xlink:title="zip">doi:10.5194/hess-21-779-2017-supplement</inline-supplementary-material>.</bold><?xmltex \hack{\vspace*{-6mm}}?></p></supplementary-material>
        </app-group><notes notes-type="authorcontribution">

      <p>Ruud J. van der Ent and Obbe A. Tuinenburg designed the study,
performed the analysis and wrote the paper.</p>
  </notes><notes notes-type="competinginterests">

      <p>The authors declare that they have no conflict of interest.</p>
  </notes><ack><title>Acknowledgements</title><p>We would like to acknowledge ECMWF for supplying ERA-Interim data through
their server at <uri>http://www.ecmwf.int</uri>. We thank Niek van de Koppel and
Tolga Cömert from Delft University of Technology for the translation of the
code of WAM-2layers from Matlab to Python, which has been used for this study.
Furthermore, we thank Patrick Keys of Stockholm University for comments on
the HESSD version of the paper. Moreover, we would like to thank the editor
and everyone that has participated in the lively interactive discussion.
Ruud J. van der Ent received funding from the European Union Seventh Framework
Programme (FP7/2007–2013) under grant agreement no. 603608, Global Earth
Observation for integrated water resource assessment: eartH2Observe. The
views expressed herein are those of the authors and do not necessarily
reflect those of the European Commission. <?xmltex \hack{\newline}?><?xmltex \hack{\newline}?>
Edited by: H. Cloke <?xmltex \hack{\newline}?>
Reviewed by: K. Trenberth, J. Wei, and two anonymous referees</p></ack><ref-list>
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<abstract-html><p class="p">This paper revisits the knowledge on the residence time of water in the
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ways of looking at temporal characteristics of atmospheric water. Longer
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high precipitation. From our analysis we find that the residence time over
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the characteristics of the turnover of water in the atmosphere in time and
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